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000028617 084__ $$2WoS$$aChemistry, Analytical
000028617 084__ $$2WoS$$aElectrochemistry
000028617 1001_ $$0P:(DE-Juel1)VDB5414$$aIbach, H.$$b0$$uFZJ
000028617 245__ $$aPotential dependence of the step line tension on surfaces in contact with an electrolyte
000028617 260__ $$aNew York, NY [u.a.]$$bElsevier$$c2003
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000028617 440_0 $$03261$$aJournal of Electroanalytical Chemistry$$v544$$x0022-0728
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000028617 520__ $$aThe potential dependence of the step line tension for electrodes in contact with an electrolyte, but without specific adsorption, is calculated by solving the Poisson-Boltzmann equation numerically. Two contributions to the potential dependence are found. A contribution arising from the step geometry is zero at the potential of zero charge (pzc) and positive for either sign of the potential. The prevailing contribution arises from the dipole moment of the charge distribution at steps. It is approximately proportional to the dipole moment and the specific surface charge, and negative for potentials positive of pzc. (C) 2003 Published by Elsevier Science B.V.
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000028617 65320 $$2Author$$asingle-crystal electrode
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000028617 65320 $$2Author$$ainterfacial structure
000028617 65320 $$2Author$$atension
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000028617 7001_ $$0P:(DE-Juel1)4744$$aGiesen, M.$$b1$$uFZJ
000028617 7001_ $$0P:(DE-HGF)0$$aSchmickler, W.$$b2
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000028617 9201_ $$0I:(DE-Juel1)VDB43$$d31.12.2006$$gISG$$kISG-3$$lInstitut für Grenzflächen und Vakuumtechnologien$$x0
000028617 9201_ $$0I:(DE-Juel1)VDB44$$d31.12.2001$$gISG$$kISG-4$$lInstitut für biologisch-anorganische Grenzflächen$$x1
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