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000029246 0247_ $$2DOI$$a10.1029/2002JD002883
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000029246 084__ $$2WoS$$aMeteorology & Atmospheric Sciences
000029246 1001_ $$0P:(DE-Juel1)VDB4867$$aThompson, A.$$b0$$uFZJ
000029246 245__ $$aConcentration and Stable Carbon Isotopic Composition of Ethane and Benzene Using a Global 3D Isotope Inclusive Chemical Tracer Model
000029246 260__ $$aWashington, DC$$bUnion$$c2003
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000029246 440_0 $$06393$$aJournal of Geophysical Research D: Atmospheres$$v108$$x0148-0227$$yD13
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000029246 520__ $$aA three-dimensional global chemical tracer model of the atmosphere has been adapted to include the stable carbon isotopic composition and isotopic fractionation of ethane and benzene. For computational efficiency the chemistry was based on a prescribed OH- radical concentration field, and therefore the feedback of ethane and benzene chemistry on the atmospheric OH- radical concentrations was not considered. The Emission Database for Global Atmospheric Research (EDGAR) V2.0 emission database used needed to be scaled by a factor of 2.22 in order to have good agreement between observed and modeled concentrations. Modeled isotopic compositions were consistent with the few published observations. The global distribution of modeled stable carbon isotope ratios and the derived mean photochemical ages of ethane and benzene are presented. The model predicts distinct regimes of photochemical aging and air mass mixing for polar regions.
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000029246 65320 $$2Author$$astable carbon isotope ratios
000029246 65320 $$2Author$$anonmethane hydrocarbons
000029246 65320 $$2Author$$aethane
000029246 65320 $$2Author$$abenzene
000029246 65320 $$2Author$$amean photochemical age
000029246 7001_ $$0P:(DE-Juel1)VDB1361$$aRudolph, J.$$b1$$uFZJ
000029246 7001_ $$0P:(DE-Juel1)16347$$aRohrer, F.$$b2$$uFZJ
000029246 7001_ $$0P:(DE-Juel1)3709$$aStein, O.$$b3$$uFZJ
000029246 773__ $$0PERI:(DE-600)2016800-7 $$a10.1029/2002JD002883$$gVol. 108, p. 4373$$p4373$$q108<4373$$tJournal of geophysical research / Atmospheres  $$tJournal of Geophysical Research$$v108$$x0148-0227$$y2003
000029246 8567_ $$uhttp://dx.doi.org/10.1029/2002JD002883
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