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@ARTICLE{Thompson:29246,
author = {Thompson, A. and Rudolph, J. and Rohrer, F. and Stein, O.},
title = {{C}oncentration and {S}table {C}arbon {I}sotopic
{C}omposition of {E}thane and {B}enzene {U}sing a {G}lobal
3{D} {I}sotope {I}nclusive {C}hemical {T}racer {M}odel},
journal = {Journal of Geophysical Research},
volume = {108},
issn = {0148-0227},
address = {Washington, DC},
publisher = {Union},
reportid = {PreJuSER-29246},
pages = {4373},
year = {2003},
note = {Record converted from VDB: 12.11.2012},
abstract = {A three-dimensional global chemical tracer model of the
atmosphere has been adapted to include the stable carbon
isotopic composition and isotopic fractionation of ethane
and benzene. For computational efficiency the chemistry was
based on a prescribed OH- radical concentration field, and
therefore the feedback of ethane and benzene chemistry on
the atmospheric OH- radical concentrations was not
considered. The Emission Database for Global Atmospheric
Research (EDGAR) V2.0 emission database used needed to be
scaled by a factor of 2.22 in order to have good agreement
between observed and modeled concentrations. Modeled
isotopic compositions were consistent with the few published
observations. The global distribution of modeled stable
carbon isotope ratios and the derived mean photochemical
ages of ethane and benzene are presented. The model predicts
distinct regimes of photochemical aging and air mass mixing
for polar regions.},
keywords = {J (WoSType)},
cin = {ICG-II},
ddc = {550},
cid = {I:(DE-Juel1)VDB48},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000184002900002},
doi = {10.1029/2002JD002883},
url = {https://juser.fz-juelich.de/record/29246},
}