001     29882
005     20250129094308.0
017 _ _ |a This version is available at the following Publisher URL: http://prb.aps.org
024 7 _ |a 10.1103/PhysRevB.67.020409
|2 DOI
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024 7 _ |a 2128/1318
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037 _ _ |a PreJuSER-29882
041 _ _ |a eng
082 _ _ |a 530
084 _ _ |2 WoS
|a Physics, Condensed Matter
100 1 _ |a Campbell, B. J.
|b 0
|0 P:(DE-HGF)0
245 _ _ |a Polaronic orbital polarization in a layered colossal magnetoresistive manganite
260 _ _ |a College Park, Md.
|b APS
|c 2003
300 _ _ |a 020409
336 7 _ |a Journal Article
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440 _ 0 |a Physical Review B
|x 1098-0121
|0 4919
|v 67
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a The striking anisotropy observed in Huang scattering distributions near the intense Bragg reflections of La1.2Sr1.8Mn2O7 is shown to be the result of orbitally polarized polarons in the paramagnetic insulating state above T-C. X-ray single-crystal diffuse scattering patterns from this bilayered colossal magnetoresistive manganite are calculated in terms of the polaronic local structure and compared with experimental measurements. At 300 K, the polaronic e(g) electrons occupy "out-of-plane" (i.e., 3z(2)-r(2)) orbitals, leading to MnO6 octahedra that are Jahn-Teller elongated along the c axis, perpendicular to the perovskite layers. Between 300 K and T-C, however, the "orbital polarization" is shown to shift into the a-b plane (i.e., 3x(2)-r(2) and 3y(2)-r(2) orbitals), allowing the formation of nanoscale polaron correlations above T-C.
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542 _ _ |i 2003-01-31
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700 1 _ |a Sinha, S. K.
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700 1 _ |a Osborn, R.
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700 1 _ |a Rosenkranz, S.
|b 3
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700 1 _ |a Mitchell, J. F.
|b 4
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700 1 _ |a Argyriou, D. N.
|b 5
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700 1 _ |a Vasiliu-Doloc, L.
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700 1 _ |a Seeck, O.
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700 1 _ |a Lynn, J. W.
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773 1 8 |a 10.1103/physrevb.67.020409
|b American Physical Society (APS)
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|t Physical Review B
|v 67
|y 2003
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773 _ _ |a 10.1103/PhysRevB.67.020409
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856 7 _ |u http://dx.doi.org/10.1103/PhysRevB.67.020409
|u http://hdl.handle.net/2128/1318
856 4 _ |u https://juser.fz-juelich.de/record/29882/files/27098.pdf
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