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000030387 1001_ $$0P:(DE-HGF)0$$aMöhler, O.$$b0
000030387 245__ $$aExperimental investigation of homogeneous freezing of sulphuric acid particles in the aerosol chamber AIDA
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000030387 520__ $$aThe homogeneous freezing of supercooled H2SO4/H2O solution droplets was investigated in the aerosol chamber AIDA (Aerosol Interactions and Dynamics in the Atmosphere) of Forschungszentrum Karlsruhe. 24 freezing experiments were performed at temperatures between 189 and 235 K with aerosol particles in the diameter range 0.05 to 1 mum. Individual experiments started at homogeneous temperatures and ice saturation ratios between 0.9 and 0.95. Cloud cooling rates up to -2.8 K min(-1) were simulated dynamically in the chamber by expansion cooling using a mechanical pump. Depending on the cooling rate and starting temperature, freezing threshold relative humidities were exceeded after expansion time periods between about 1 and 10 min. The onset of ice formation was measured with three independent methods showing good agreement among each other. Ice saturation ratios measured at the onset of ice formation increased from about 1.4 at 231 K to about 1.75 at 189 K. The experimental data set including thermodynamic parameters as well as physical and chemical aerosol analysis provides a good basis for microphysical model applications.
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000030387 7001_ $$0P:(DE-HGF)0$$aStetzer, O.$$b1
000030387 7001_ $$0P:(DE-HGF)0$$aSchaefers, S.$$b2
000030387 7001_ $$0P:(DE-HGF)0$$aLinke, C.$$b3
000030387 7001_ $$0P:(DE-HGF)0$$aSchnaiter, M.$$b4
000030387 7001_ $$0P:(DE-HGF)0$$aTiede, R.$$b5
000030387 7001_ $$0P:(DE-HGF)0$$aSaathoff, H.$$b6
000030387 7001_ $$0P:(DE-Juel1)129131$$aKrämer, M.$$b7$$uFZJ
000030387 7001_ $$0P:(DE-HGF)0$$aMangold, A.$$b8
000030387 7001_ $$0P:(DE-HGF)0$$aBudz, P.$$b9
000030387 7001_ $$0P:(DE-HGF)0$$aZink, P.$$b10
000030387 7001_ $$0P:(DE-HGF)0$$aSchreiner, J.$$b11
000030387 7001_ $$0P:(DE-HGF)0$$aMauersberger, K.$$b12
000030387 7001_ $$0P:(DE-HGF)0$$aHaag, W.$$b13
000030387 7001_ $$0P:(DE-HGF)0$$aKärcher, B.$$b14
000030387 7001_ $$0P:(DE-HGF)0$$aSchurath, U.$$b15
000030387 773__ $$0PERI:(DE-600)2069847-1$$gVol. 3, p. 211 - 223$$p211 - 223$$q3<211 - 223$$tAtmospheric chemistry and physics$$v3$$x1680-7316$$y2003
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