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@ARTICLE{Mhler:30387,
author = {Möhler, O. and Stetzer, O. and Schaefers, S. and Linke, C.
and Schnaiter, M. and Tiede, R. and Saathoff, H. and
Krämer, M. and Mangold, A. and Budz, P. and Zink, P. and
Schreiner, J. and Mauersberger, K. and Haag, W. and
Kärcher, B. and Schurath, U.},
title = {{E}xperimental investigation of homogeneous freezing of
sulphuric acid particles in the aerosol chamber {AIDA}},
journal = {Atmospheric chemistry and physics},
volume = {3},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-30387},
pages = {211 - 223},
year = {2003},
note = {Record converted from VDB: 12.11.2012},
abstract = {The homogeneous freezing of supercooled H2SO4/H2O solution
droplets was investigated in the aerosol chamber AIDA
(Aerosol Interactions and Dynamics in the Atmosphere) of
Forschungszentrum Karlsruhe. 24 freezing experiments were
performed at temperatures between 189 and 235 K with aerosol
particles in the diameter range 0.05 to 1 mum. Individual
experiments started at homogeneous temperatures and ice
saturation ratios between 0.9 and 0.95. Cloud cooling rates
up to -2.8 K min(-1) were simulated dynamically in the
chamber by expansion cooling using a mechanical pump.
Depending on the cooling rate and starting temperature,
freezing threshold relative humidities were exceeded after
expansion time periods between about 1 and 10 min. The onset
of ice formation was measured with three independent methods
showing good agreement among each other. Ice saturation
ratios measured at the onset of ice formation increased from
about 1.4 at 231 K to about 1.75 at 189 K. The experimental
data set including thermodynamic parameters as well as
physical and chemical aerosol analysis provides a good basis
for microphysical model applications.},
keywords = {J (WoSType)},
cin = {ICG-I},
ddc = {550},
cid = {I:(DE-Juel1)VDB47},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000181074900002},
url = {https://juser.fz-juelich.de/record/30387},
}