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000030847 084__ $$2WoS$$aChemistry, Physical
000030847 084__ $$2WoS$$aPhysics, Condensed Matter
000030847 1001_ $$0P:(DE-Juel1)VDB5414$$aIbach, H.$$b0$$uFZJ
000030847 245__ $$aThe instability of vicinal electrode surfaces against step bunching II : theory
000030847 260__ $$aAmsterdam$$bElsevier$$c2004
000030847 300__ $$a24 - 31
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000030847 520__ $$aIt is shown that vicinal surfaces with a regular step array in contact with an electrolyte are intrinsically unstable against a phase separation into areas of flat terraces and areas of step bunches. The effect is caused by the step dipole moment which lowers the potential of zero charge (pzc) of stepped surfaces. Specific calculations performed for vicinal surfaces of silver are qualitatively in keeping with experimental observations. Step bunching is likewise expected for vicinal surfaces of gold and platinum. (C) 2004 Elsevier B.V. All rights reserved.
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000030847 65320 $$2Author$$avicinal single crystal surfaces
000030847 65320 $$2Author$$asurface thermodynamics (including phase transitions)
000030847 65320 $$2Author$$asurface tension
000030847 65320 $$2Author$$asolid-liquid interfaces
000030847 7001_ $$0P:(DE-HGF)0$$aSchmickler, W.$$b1
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