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@ARTICLE{Staikov:31348,
      author       = {Staikov, G. and Kunze, J. and Strehblow, H.-H.},
      title        = {{I}n situ {STM} {S}tudy of the {I}nitial {S}tages of
                      {E}lectrochemical {O}xide {F}ormation at the
                      {A}g(111)/0.1{M} {N}a{OH}(aq) {I}nterface},
      journal      = {Electrochemistry communications},
      volume       = {6},
      issn         = {1388-2481},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier Science},
      reportid     = {PreJuSER-31348},
      pages        = {132 - 137},
      year         = {2004},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The atomic structure of surface layers and the local
                      changes of surface morphology during the initial stages of
                      anodic oxidation of Ag(111) in an aqueous 0.1 M NaOH
                      solution have been investigated by in situ scanning
                      tunneling microscopy (STM) under different polarization
                      conditions. The surface oxide formation starts at
                      underpotentials, i.e. at electrode potentials E below the
                      Nernst-potential E-3DAg2O (vs. SHE) = 0.4 V for the
                      formation of the three-dimensional (3D) bulk Ag2O phase. An
                      ordered overlayer showing distinct Moire pattern is observed
                      in the potential range -0.1 V < E (vs. SHE) < 0.1 V. The
                      appearance of the Moire structure is assigned to the strong
                      OH adsorption, which induces a stretching of the 2D lattice
                      of the OH-terminated topmost Ag(111) monolayer. In situ STM
                      imaging at higher potentials (0.1 V < E (vs. SHE) < 0.3 V)
                      shows the occurrence of a Ag dissolution process followed by
                      an underpotential oxide formation in agreement with previous
                      electrochemical measurements and in situ X-ray absorption
                      studies. (C) 2003 Elsevier B.V. All rights reserved.},
      keywords     = {J (WoSType)},
      cin          = {ISG-3},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB43},
      pnm          = {Kondensierte Materie},
      pid          = {G:(DE-Juel1)FUEK242},
      shelfmark    = {Electrochemistry},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000188507400007},
      doi          = {10.1016/j.elecom.2003.10.027},
      url          = {https://juser.fz-juelich.de/record/31348},
}