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000032153 084__ $$2WoS$$aChemistry, Physical
000032153 1001_ $$0P:(DE-Juel1)VDB22267$$aNagy, G.$$b0$$uFZJ
000032153 245__ $$aAdlayer Structures Probed by Distance Tunneling Spectroscopy for Au(111)/H2SO4   Cu2
000032153 260__ $$aMünchen$$bOldenbourg$$c2003
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000032153 520__ $$aWe performed a series of distance tunnelling characteristics measurements for the system Au(111)/0.05 M H2SO4 + 1 mM Cu2+ to understand, if it is possible to map the liquid part of the double layer perpendicular to the electrode surface. We found that we probed the double layer in a distance range where we do not penetrate into the inner Helmholtz layer. Nevertheless, the tip is sufficiently close to the metal surface to address adlayer features showing sensitivity toward long-range ordered structures. The bias between the STM tip and the sample drops in the inner Helmholtz layer, and electronic overlap exists between the adsorbed layer and the metal surface. Molecular contributions to the electronic structure of ordered adlayers appear to be detectable. At larger distances from the surface the average barrier height was found to be about 1 eV, practically independent on the electrode potential.
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000032153 65320 $$2Author$$adouble layer
000032153 65320 $$2Author$$aSTM
000032153 65320 $$2Author$$aSTS
000032153 65320 $$2Author$$abarrier height
000032153 65320 $$2Author$$aCuUPD
000032153 65320 $$2Author$$aanions
000032153 65320 $$2Author$$aAu(111)
000032153 7001_ $$0P:(DE-Juel1)VDB5443$$aWandlowski, T.$$b1$$uFZJ
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