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@ARTICLE{Nagy:32153,
      author       = {Nagy, G. and Wandlowski, T.},
      title        = {{A}dlayer {S}tructures {P}robed by {D}istance {T}unneling
                      {S}pectroscopy for {A}u(111)/{H}2{SO}4 {C}u2},
      journal      = {Zeitschrift für Physikalische Chemie},
      volume       = {217},
      issn         = {0942-9352},
      address      = {München},
      publisher    = {Oldenbourg},
      reportid     = {PreJuSER-32153},
      pages        = {587 - 605},
      year         = {2003},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {We performed a series of distance tunnelling
                      characteristics measurements for the system Au(111)/0.05 M
                      H2SO4 + 1 mM Cu2+ to understand, if it is possible to map
                      the liquid part of the double layer perpendicular to the
                      electrode surface. We found that we probed the double layer
                      in a distance range where we do not penetrate into the inner
                      Helmholtz layer. Nevertheless, the tip is sufficiently close
                      to the metal surface to address adlayer features showing
                      sensitivity toward long-range ordered structures. The bias
                      between the STM tip and the sample drops in the inner
                      Helmholtz layer, and electronic overlap exists between the
                      adsorbed layer and the metal surface. Molecular
                      contributions to the electronic structure of ordered
                      adlayers appear to be detectable. At larger distances from
                      the surface the average barrier height was found to be about
                      1 eV, practically independent on the electrode potential.},
      keywords     = {J (WoSType)},
      cin          = {ISG-3},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB43},
      pnm          = {Materialien, Prozesse und Bauelemente für die Mikro- und
                      Nanoelektronik},
      pid          = {G:(DE-Juel1)FUEK252},
      shelfmark    = {Chemistry, Physical},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000182884100010},
      doi          = {10.1524/zpch.217.5.587.20456},
      url          = {https://juser.fz-juelich.de/record/32153},
}