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| 001 | 32207 | ||
| 005 | 20180210134731.0 | ||
| 024 | 7 | _ | |2 DOI |a 10.1016/S0013-4686(02)00836-8 |
| 024 | 7 | _ | |2 WOS |a WOS:000181814400018 |
| 037 | _ | _ | |a PreJuSER-32207 |
| 041 | _ | _ | |a eng |
| 082 | _ | _ | |a 540 |
| 084 | _ | _ | |2 WoS |a Electrochemistry |
| 100 | 1 | _ | |a García, S. G. |b 0 |0 P:(DE-HGF)0 |
| 245 | _ | _ | |a STM Tip-Induced Local Electrochemical Dissolution of Silver |
| 260 | _ | _ | |a New York, NY [u.a.] |b Elsevier |c 2003 |
| 300 | _ | _ | |a 1279 - 1285 |
| 336 | 7 | _ | |a Journal Article |0 PUB:(DE-HGF)16 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a JOURNAL_ARTICLE |2 ORCID |
| 336 | 7 | _ | |a article |2 DRIVER |
| 440 | _ | 0 | |a Electrochimica Acta |x 0013-4686 |0 1776 |v 48 |
| 500 | _ | _ | |a Record converted from VDB: 12.11.2012 |
| 520 | _ | _ | |a Local dissolution/deposition processes under in situ scanning tunneling microscopy (STM) imaging conditions are studied in the systems Ag(111)/Ag+, ClO4- and Ag(111)/Ag+, SO42-. The results show that in both systems the local kinetics of these processes strongly depend on the polarization conditions. At STM-tip potentials more positive than the Ag/Ag+ equilibrium potential, a local dissolution of the Ag(111) substrate is observed even at cathodic substrate overpotentials at which the overall substrate current density is cathodic. This tip-induced Ag dissolution is in agreement with results obtained recently in the system Cu((111))/Cu2+. The enhanced local Ag dissolution is explained by a reduced Ag+ concentration underneath the STM tip promoted by both an electrostatic repulsion of Ag+ and a reduction of the mass transport due to the shielding effect of the tip. The possibility for a preparation of negative Ag nanostructures by STM tip-induced electrochemical dissolution is demonstrated. (C) 2003 Elsevier Science Ltd. All rights reserved. |
| 536 | _ | _ | |a Materialien, Prozesse und Bauelemente für die Mikro- und Nanoelektronik |c I01 |2 G:(DE-HGF) |0 G:(DE-Juel1)FUEK252 |x 0 |
| 588 | _ | _ | |a Dataset connected to Web of Science |
| 650 | _ | 7 | |a J |2 WoSType |
| 653 | 2 | 0 | |2 Author |a silver |
| 653 | 2 | 0 | |2 Author |a STM |
| 653 | 2 | 0 | |2 Author |a tip-induced dissolution |
| 653 | 2 | 0 | |2 Author |a local etching |
| 653 | 2 | 0 | |2 Author |a nanostructuring |
| 700 | 1 | _ | |a Salinas, D. R. |b 1 |0 P:(DE-HGF)0 |
| 700 | 1 | _ | |a Mayer, C. E. |b 2 |0 P:(DE-HGF)0 |
| 700 | 1 | _ | |a Lorenz, W. J. |b 3 |0 P:(DE-HGF)0 |
| 700 | 1 | _ | |a Staikov, G. |b 4 |u FZJ |0 P:(DE-Juel1)VDB13645 |
| 773 | _ | _ | |a 10.1016/S0013-4686(02)00836-8 |g Vol. 48, p. 1279 - 1285 |p 1279 - 1285 |q 48<1279 - 1285 |0 PERI:(DE-600)1483548-4 |t Electrochimica acta |v 48 |y 2003 |x 0013-4686 |
| 856 | 7 | _ | |u http://dx.doi.org/10.1016/S0013-4686(02)00836-8 |
| 909 | C | O | |o oai:juser.fz-juelich.de:32207 |p VDB |
| 913 | 1 | _ | |k I01 |v Materialien, Prozesse und Bauelemente für die Mikro- und Nanoelektronik |l Informationstechnologie mit nanoelektronischen Systemen |b Information |0 G:(DE-Juel1)FUEK252 |x 0 |
| 914 | 1 | _ | |y 2003 |
| 915 | _ | _ | |0 StatID:(DE-HGF)0010 |a JCR/ISI refereed |
| 920 | 1 | _ | |k ISG-3 |l Institut für Grenzflächen und Vakuumtechnologien |d 31.12.2006 |g ISG |0 I:(DE-Juel1)VDB43 |x 0 |
| 970 | _ | _ | |a VDB:(DE-Juel1)34033 |
| 980 | _ | _ | |a VDB |
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| 980 | _ | _ | |a journal |
| 980 | _ | _ | |a I:(DE-Juel1)PGI-3-20110106 |
| 980 | _ | _ | |a UNRESTRICTED |
| 981 | _ | _ | |a I:(DE-Juel1)PGI-3-20110106 |
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