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| Hauptseite > Publikationsdatenbank > Charge transport in single Au-Alkandithiol-Au junctions - Conductance histograms and conformational degress of freedom > print |
| Hauptseite > Publikationsdatenbank > Charge transport in single Au-Alkandithiol-Au junctions - Conductance histograms and conformational degress of freedom > print |
| 001 | 329 | ||
| 005 | 20200731122043.0 | ||
| 024 | 7 | _ | |a pmid:18076172 |2 pmid |
| 024 | 7 | _ | |a 10.1021/ja0762386 |2 DOI |
| 024 | 7 | _ | |a WOS:000252127500053 |2 WOS |
| 024 | 7 | _ | |a 2128/25409 |2 Handle |
| 037 | _ | _ | |a PreJuSER-329 |
| 041 | _ | _ | |a eng |
| 082 | _ | _ | |a 540 |
| 084 | _ | _ | |2 WoS |a Chemistry, Multidisciplinary |
| 100 | 1 | _ | |a Li, C. |b 0 |u FZJ |0 P:(DE-Juel1)VDB63965 |
| 245 | _ | _ | |a Charge transport in single Au-Alkandithiol-Au junctions - Conductance histograms and conformational degress of freedom |
| 260 | _ | _ | |a Washington, DC |b American Chemical Society |c 2008 |
| 300 | _ | _ | |a 318 - 326 |
| 336 | 7 | _ | |a Journal Article |0 PUB:(DE-HGF)16 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
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| 336 | 7 | _ | |a article |2 DRIVER |
| 440 | _ | 0 | |a Journal of the American Chemical Society |x 0002-7863 |0 8502 |v 130 |
| 500 | _ | _ | |a Record converted from VDB: 12.11.2012 |
| 520 | _ | _ | |a Recent STM molecular break-junction experiments have revealed multiple series of peaks in the conductance histograms of alkanedithiols. To resolve a current controversy, we present here an in-depth study of charge transport properties of Au|alkanedithiol|Au junctions. Conductance histograms extracted from our STM measurements unambiguously confirm features showing more than one set of junction configurations. On the basis of quantum chemistry calculations, we propose that certain combinations of different sulfur-gold couplings and trans/gauche conformations act as the driving agents. The present study may have implications for experimental methodology: whenever conductances of different junction conformations are not statistically independent, the conductance histogram technique can exhibit a single series only, even though a much larger abundance of microscopic realizations exists. |
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| 650 | _ | 2 | |2 MeSH |a Electric Conductivity |
| 650 | _ | 2 | |2 MeSH |a Gold: chemistry |
| 650 | _ | 2 | |2 MeSH |a Molecular Conformation |
| 650 | _ | 2 | |2 MeSH |a Quantum Theory |
| 650 | _ | 2 | |2 MeSH |a Sulfhydryl Compounds: chemistry |
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| 650 | _ | 7 | |0 7440-57-5 |2 NLM Chemicals |a Gold |
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| 700 | 1 | _ | |a Pobelov, I. |b 1 |u FZJ |0 P:(DE-Juel1)VDB45469 |
| 700 | 1 | _ | |a Wandlowski, Th. |b 2 |u FZJ |0 P:(DE-Juel1)VDB9859 |
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| 700 | 1 | _ | |a Arnold, A. |b 4 |0 P:(DE-HGF)0 |
| 700 | 1 | _ | |a Evers, F. |b 5 |0 P:(DE-HGF)0 |
| 773 | _ | _ | |a 10.1021/ja0762386 |g Vol. 130, p. 318 - 326 |p 318 - 326 |q 130<318 - 326 |0 PERI:(DE-600)1472210-0 |t Journal of the American Chemical Society |v 130 |y 2008 |x 0002-7863 |
| 856 | 7 | _ | |u http://dx.doi.org/10.1021/ja0762386 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/329/files/0802.2407.pdf |y OpenAccess |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/329/files/0802.2407.pdf?subformat=pdfa |x pdfa |y OpenAccess |
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