001     33294
005     20240712101001.0
024 7 _ |a 10.1029/2000JD000136
|2 DOI
024 7 _ |a WOS:000180427400006
|2 WOS
024 7 _ |a 0022-1406
|2 ISSN
024 7 _ |a 0148-0227
|2 ISSN
024 7 _ |a 2128/20617
|2 Handle
037 _ _ |a PreJuSER-33294
041 _ _ |a eng
082 _ _ |a 550
082 _ _ |a 550
084 _ _ |2 WoS
|a Meteorology & Atmospheric Sciences
100 1 _ |a Balis, D.
|b 0
|0 P:(DE-HGF)0
245 _ _ |a Measurements and modeling of photolysis rates during the Photochemical Activity and Ultraviolet Radiation (PAUR) II campaign
260 _ _ |a Washington, DC
|b Union
|c 2002
|a Washington, DC
|b Union
295 1 0 |a .
300 _ _ |a PAU 5-1 - PAU 5-12
336 7 _ |a Journal Article
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336 7 _ |a Output Types/Journal article
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336 7 _ |a Journal Article
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336 7 _ |a ARTICLE
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336 7 _ |a article
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440 _ 0 |a Journal of Geophysical Research
|x 0022-1406
|0 3369
|y D18
|v 107
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a [1] In this paper we compare radiative transfer model calculations of the actinic flux in the UV spectral region with airborne measurements of the actinic flux, obtained during the Photochemical Activity and Ultraviolet Radiation (PAUR) campaign, which took place in the Aegean Sea, Greece, in June 1996, in order to assess the accuracy of the model in calculating photolysis rates, when the model input parameters are well defined from measurements. The model can simulate the total actinic flux (4 pi sr) in the UV-A region with an accuracy of 5% for all altitudes (0.1-12 km) in the cloud free troposphere, while in the UV-B the impact of the vertical distribution of ozone and aerosol can lead to differences, of about 5-10% at low altitudes up to 20% at higher altitudes. Next, the photolysis rates of J((OD)-D-1) and J(NO2) measured during the PAUR 2, in Crete, Greece (35.5degreesN, 23.8degreesE), in May 1999, at two altitudes (Gerani 30 m and Prases 1000 m), are compared with the respective model calculations in order to examine the effect of the alternating Sahara dust/maritime aerosol environments imposed to these photolysis rates, as well as to examine their differences due to the altitude difference. It is shown that high levels of tropospheric ozone and absorbing aerosols can cause a decrease in the photolysis rates of ozone near the surface, even under conditions of reduced total ozone content. This fact indicates that tropospheric ozone can be disproportionately important as a filter against UV-B radiation when most scattering of the radiation by air molecules and dust occurs in the troposphere. This behavior is not simulated accurately using a radiative transfer model constrained by observations of ozone and aerosol optical depths. The differences of the of the photolysis rates between the two altitudes as determined by the model and by the measurements, differ significantly for the Sahara dust event, indicating that during this event in the boundary layer, there is a mixture of desert and nonabsorbing aerosols.
536 _ _ |a Chemie und Dynamik der Geo-Biosphäre
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650 _ 7 |a J
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653 2 0 |2 Author
|a total ozone
653 2 0 |2 Author
|a photochemistry
653 2 0 |2 Author
|a UVB radiation
700 1 _ |a Zerefos, C. S.
|b 1
|0 P:(DE-HGF)0
700 1 _ |a Kourtidis, K.
|b 2
|0 P:(DE-HGF)0
700 1 _ |a Bais, A. F.
|b 3
|0 P:(DE-HGF)0
700 1 _ |a Hofzumahaus, A.
|b 4
|u FZJ
|0 P:(DE-Juel1)16326
700 1 _ |a Kraus, A.
|b 5
|u FZJ
|0 P:(DE-Juel1)VDB832
700 1 _ |a Schmitt, R.
|b 6
|0 P:(DE-HGF)0
700 1 _ |a Blumthaler, M.
|b 7
|0 P:(DE-HGF)0
700 1 _ |a Gobbi, G. P.
|b 8
|0 P:(DE-HGF)0
773 _ _ |0 PERI:(DE-600)2016800-7
|a 10.1029/2000JD000136
|g Vol. 107, p. PAU 5-1 - PAU 5-12
|p PAU 5-1 - PAU 5-12
|q 107|t Journal of geophysical research / Atmospheres
|v 107
|x 0022-1406
|y 2002
856 7 _ |u http://dx.doi.org/10.1029/2000JD000136
856 4 _ |u https://juser.fz-juelich.de/record/33294/files/2000JD000136.pdf
|y OpenAccess
856 4 _ |u https://juser.fz-juelich.de/record/33294/files/2000JD000136.pdf?subformat=pdfa
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913 1 _ |k U01
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914 1 _ |y 2002
915 _ _ |a OpenAccess
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915 _ _ |a JCR/ISI refereed
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920 1 _ |k ICG-II
|l Troposphäre
|d 31.12.2006
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981 _ _ |a I:(DE-Juel1)IEK-8-20101013


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