TY - JOUR AU - Elfrink, K. AU - Ollesch, J. AU - Stoehr, J. AU - Willbold, D. AU - Riesner, D. AU - Gerwert, K. TI - Structural changes of membrane-anchored native PrPc JO - Proceedings of the National Academy of Sciences of the United States of America VL - 105 SN - 0027-8424 CY - Washington, DC PB - Academy M1 - PreJuSER-340 SP - 10815 - 10819 PY - 2008 N1 - Record converted from VDB: 12.11.2012 AB - Misfolding and subsequent aggregation of endogenous proteins constitute essential steps in many human disorders, including Alzheimer and prion diseases. In most prion protein-folding studies, the posttranslational modifications, the lipid anchor in particular, were lacking. Here, we studied a fully posttranslationally modified cellular prion protein, carrying two N-glycosylations and the natural GPI anchor. We used time-resolved FTIR to study the prion protein secondary structure changes when binding to a raft-like lipid membrane via its GPI anchor. We observed that membrane anchoring above a threshold concentration induced refolding of the prion protein to intermolecular beta-sheets. Such transition is not observed in solution and is membrane specific. Excessive membrane anchoring, analyzed with molecular sensitivity, is thought to be a crucial event in the development of prion diseases. KW - Animals KW - Cricetinae KW - Membrane Proteins: genetics KW - Mesocricetus KW - Models, Molecular KW - PrPC Proteins: genetics KW - Protein Conformation KW - Protein Folding KW - Spectroscopy, Fourier Transform Infrared KW - Membrane Proteins (NLM Chemicals) KW - PrPC Proteins (NLM Chemicals) KW - J (WoSType) LB - PUB:(DE-HGF)16 C6 - pmid:18669653 C2 - pmc:PMC2504809 UR - <Go to ISI:>//WOS:000258308500036 DO - DOI:10.1073/pnas.0804721105 UR - https://juser.fz-juelich.de/record/340 ER -