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000034038 0247_ $$2DOI$$a10.1103/PhysRevLett.91.165701
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000034038 084__ $$2WoS$$aPhysics, Multidisciplinary
000034038 1001_ $$0P:(DE-Juel1)VDB293$$aDogic, Z.$$b0$$uFZJ
000034038 245__ $$aSurface Freezing and a Two-Step Pathway of the Isotropic-Smectic Phase Transition in Colloidal Rods
000034038 260__ $$aCollege Park, Md.$$bAPS$$c2003
000034038 300__ $$a165701-1 - 165701-4
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000034038 440_0 $$04925$$aPhysical Review Letters$$v91$$x0031-9007$$y16
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000034038 520__ $$aWe study the kinetics of the isotropic-smectic phase transition in a colloidal rod/polymer mixture by visualizing individual smectic layers. First, we show that the bulk isotropic-smectic phase transition is preceded by a surface freezing transition in which a quasi-two-dimensional smectic phase wets the isotropic-nematic interface. Next, we identify a two-step kinetic pathway for the formation of a bulk smectic phase. In the first step a metastable isotropic-nematic interface is formed. This interface is wetted by the surface-induced smectic phase. In the subsequent step, smectic layers nucleate at this surface phase and grow into the isotropic bulk phase.
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000034038 8567_ $$uhttp://hdl.handle.net/2128/1622$$uhttp://dx.doi.org/10.1103/PhysRevLett.91.165701
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