TY - JOUR AU - Guo, X. AU - Ding, Y. TI - Grain boundary space charge effect in Zirconia JO - Journal of the Electrochemical Society VL - 151 SN - 0013-4651 CY - Pennington, NJ PB - Electrochemical Society M1 - PreJuSER-34062 SP - J1 - J7 PY - 2004 N1 - Record converted from VDB: 12.11.2012 AB - According to the space charge concept, oxygen vacancies are depleted in the grain boundary space charge layers of acceptor-doped ZrO2; whereas electrons are expected to accumulate in the space charge layers if present, leading to significant changes in the grain boundary electrical properties. In this work, electrons were introduced to 8 mol % TiO2 and 7.36 mol % Y2O3-codoped ZrO2 by annealing in the mixture of 2% H-2-Ar; as a result, the grain boundary arc disappeared, and the electrical conductivities increased considerably, especially for the sample with finer grain size. Both phenomena suggest highly conductive grain boundaries resulting from the accumulation of electrons in the space charge layers. (C) 2003 The Electrochemical Society. KW - J (WoSType) LB - PUB:(DE-HGF)16 UR - <Go to ISI:>//WOS:000187428800073 DO - DOI:10.1149/1.1625948 UR - https://juser.fz-juelich.de/record/34062 ER -