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000034172 1001_ $$0P:(DE-Juel1)VDB4228$$aFrielinghaus, H.$$b0$$uFZJ
000034172 245__ $$aBlends of AB/BC diblock copolymers with a large interaction parameter Chi
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000034172 520__ $$aBlends of poly(styrene)-b-poly(isoprene) (PS-PI) and poly( isoprene)-b-poly(ethylene oxide) (PI-PEO) were investigated by small-angle X-ray scattering, photon correlation spectroscopy, light microscopy, and rheology. Blends were prepared in which both diblocks had the same PI composition, f, and were investigated as a function of blend composition, Phi. We generally found a disordered one-phase region at high temperatures and two macrophase-separated, ordered phases at low temperatures. At low temperatures the only appreciable miscibility was found for f = 0.7 in the PI-PEO-rich phase. At intermediate temperatures we generally observed macrophase separation before microphase separation upon cooling. The macrophase separation boundary compared to the microphase boundary is lowered upon increasing f. For f = 0.6 and 0.7 we observe an adjustment of the d spacing of the macrophase-separated, ordered phases. The general trend of the phase behavior is described by a theory using the random phase approximation.
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000034172 7001_ $$0P:(DE-HGF)0$$aHermsdorf, N.$$b1
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000034172 7001_ $$0P:(DE-HGF)0$$aAlmdal, K.$$b3
000034172 7001_ $$0P:(DE-HGF)0$$aMortensen, K.$$b4
000034172 7001_ $$0P:(DE-HGF)0$$aHamley, I. W.$$b5
000034172 7001_ $$0P:(DE-HGF)0$$aMessé, L.$$b6
000034172 7001_ $$0P:(DE-HGF)0$$aCorvazier, M. F.$$b7
000034172 7001_ $$0P:(DE-HGF)0$$aRyan, A. J.$$b8
000034172 7001_ $$0P:(DE-Juel1)129425$$avan Dusschoten, D.$$b9$$uFZJ
000034172 7001_ $$0P:(DE-HGF)0$$aWilhelm, M.$$b10
000034172 7001_ $$0P:(DE-HGF)0$$aFloudas, G.$$b11
000034172 7001_ $$0P:(DE-HGF)0$$aFytas, G.$$b12
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