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@ARTICLE{Sillman:34362,
      author       = {Sillman, S. and Vautard, R. and Menut, L. and Kley, D.},
      title        = {{O}3-{NO}x-{VOC} sensitivity of {NO}x-{VOC} indicators in
                      {P}aris : results from models and {ESQUIF} measurements},
      journal      = {Journal of Geophysical Research},
      volume       = {108},
      issn         = {0148-0227},
      address      = {Washington, DC},
      publisher    = {Union},
      reportid     = {PreJuSER-34362},
      pages        = {17},
      year         = {2003},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {[1] A three-dimensional photochemical model has been used
                      to interpret aircraft measurements from the Atmospheric
                      Pollution Over the Paris Area campaign near Paris, with
                      special attention to measurements that are related to
                      predicted O-3-NOx-volatile organic compound (VOC)
                      sensitivity. The model (CHIMERE) includes a representation
                      of ozone formation over Europe and a more detailed spatial
                      representation of the region around Paris. A series of model
                      scenarios were developed with varying wind speeds and
                      emission rates. Comparisons are shown with measured O-3,
                      total reactive nitrogen (NOy), summed VOCs, and isoprene.
                      Results show that model NOx-VOC sensitivity predictions are
                      correlated with the ratio O-3/NOy but not with
                      O-3/peroxyacetyl nitrate. Measured O-3 and NOy on high-ozone
                      days tends to agree with model values when models predict
                      NOx-sensitive or transitional chemistry but not when models
                      predict VOC-sensitive chemistry. Model values for O-3/NOy
                      and the O-3-NOy slope are lower than measured values,
                      suggesting the possibility of missing, unmeasured VOCs in
                      the Paris plume. Standard performance tests for ozone
                      models, such as normalized bias, show good agreement between
                      models and measurements, even in cases when significant
                      differences appear in the O-3-NOy correlation. Model
                      predictions shift slightly toward NOx-sensitive chemistry
                      when model wind speeds are increased. Isoprene represents
                      $20\%$ of total VOC reactivity - weighted carbon in the
                      center of the Paris plume and $50\%$ in the surrounding
                      rural area during high-ozone events.},
      keywords     = {J (WoSType)},
      cin          = {ICG-II},
      ddc          = {550},
      cid          = {I:(DE-Juel1)VDB48},
      pnm          = {Chemie und Dynamik der Geo-Biosphäre},
      pid          = {G:(DE-Juel1)FUEK257},
      shelfmark    = {Meteorology $\&$ Atmospheric Sciences},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000183744400001},
      doi          = {10.1029/2002JD001561},
      url          = {https://juser.fz-juelich.de/record/34362},
}