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024 7 _ |2 DOI
|a 10.1023/A:1015709214016
024 7 _ |2 WOS
|a WOS:000175947400020
037 _ _ |a PreJuSER-34365
041 _ _ |a eng
082 _ _ |a 540
084 _ _ |2 WoS
|a Environmental Sciences
084 _ _ |2 WoS
|a Meteorology & Atmospheric Sciences
100 1 _ |a Winkler, J.
|b 0
|0 P:(DE-HGF)0
245 _ _ |a Ground-based and airborne measurements of nonmethane hydrocarbons in BERLIOZ : analysis and selected results
260 _ _ |a Dordrecht [u.a.]
|b Springer Science + Business Media B.V
|c 2002
300 _ _ |a 465 - 492
336 7 _ |a Journal Article
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336 7 _ |a Journal Article
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336 7 _ |a ARTICLE
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336 7 _ |a JOURNAL_ARTICLE
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336 7 _ |a article
|2 DRIVER
440 _ 0 |a Journal of Atmospheric Chemistry
|x 0167-7764
|0 3073
|v 42
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a During the Berlin Ozone Experiment BERLIOZ in July-August 1998 quasi-continuous measurements of C-2-C-12 nonmethane hydrocarbons (NMHCs) were carried out at 10 sites in and around the city of Berlin using on-line gas-chromatographic systems (GCs) with a temporal resolution of 20-120 minutes. Additional airborne NMHC measurements were made using canister sampling on three aircraft and an on-line GC system on a fourth aircraft. The ground based data are analyzed to characterize the different sites and to identify the influence of emissions from Berlin on its surroundings. Benzene mixing ratios at the 4 rural sites were rather low (<0.5 ppbv). Berlin (and the surrounding highway ring) was identified as the main source of anthropogenic NMHCs at Eichstadt and Blossin, whilst other sources were important at the furthermost site Menz. The median toluene/benzene concentration ratio in Berlin was 2.3 ppbv/ppbv, agreeing well with measurements in other German cities. As expected, the ratios at the background sites decreased with increasing distance to Berlin and were usually around one or below. On 20 and 21 July, the three northwesterly sites were situated downwind of Berlin and thus were influenced by its emissions. Considering the distance between the sites and the windspeed, the city plume was observed at reasonable time scales, showing decreasing toluene/benzene ratios of 2.3, 1.6 and 1.3 with increasing distance from Berlin. Isoprene was the only biogenic NMHC measured at BERLIOZ. It was the most abundant compound at the background sites on the hotter days, dominating the local NMHC reactivity with averaged contributions to the total OH loss rate of 51% and 70% at Pabstthum and Blossin, respectively. Emission ratios (relative to CO and to the sum of analysed NMHCs) were derived from airborne measurements. The comparison with an emission inventory suggests traffic-related emissions to be the predominating source of the considered hydrocarbon species. Problems were identified with the emission inventory for propane, ethene and pentanes.
536 _ _ |a Chemie und Dynamik der Geo-Biosphäre
|c U01
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588 _ _ |a Dataset connected to Web of Science
650 _ 7 |a J
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653 2 0 |2 Author
|a nonmethane hydrocarbons
653 2 0 |2 Author
|a pollution roses
653 2 0 |2 Author
|a toluene/benzene ratio
653 2 0 |2 Author
|a city plume
653 2 0 |2 Author
|a isoprene
653 2 0 |2 Author
|a NMHC/CO ratios
653 2 0 |2 Author
|a emission inventory
700 1 _ |a Blank, P.
|b 1
|0 P:(DE-HGF)0
700 1 _ |a Glaser, K.
|b 2
|0 P:(DE-HGF)0
700 1 _ |a Gomes, J. A. G.
|b 3
|0 P:(DE-HGF)0
700 1 _ |a Habram, M.
|b 4
|0 P:(DE-HGF)0
700 1 _ |a Jambert, C.
|b 5
|0 P:(DE-HGF)0
700 1 _ |a Jaeschke, W.
|b 6
|0 P:(DE-HGF)0
700 1 _ |a Konrad, S.
|b 7
|u FZJ
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700 1 _ |a Kurtenbach, R.
|b 8
|0 P:(DE-HGF)0
700 1 _ |a Lenschow, P.
|b 9
|0 P:(DE-HGF)0
700 1 _ |a Lörzer, J. C.
|b 10
|0 P:(DE-HGF)0
700 1 _ |a Perros, P. E.
|b 11
|0 P:(DE-HGF)0
700 1 _ |a Pesch, M.
|b 12
|0 P:(DE-HGF)0
700 1 _ |a Prümke, H. J.
|b 13
|0 P:(DE-HGF)0
700 1 _ |a Rappenglück, B.
|b 14
|0 P:(DE-HGF)0
700 1 _ |a Schmitz, T.
|b 15
|u FZJ
|0 P:(DE-Juel1)VDB1445
700 1 _ |a Slemr, E. C.
|b 16
|0 P:(DE-HGF)0
700 1 _ |a Volz-Thomas, A.
|b 17
|u FZJ
|0 P:(DE-Juel1)6742
700 1 _ |a Wickert, B.
|b 18
|0 P:(DE-HGF)0
773 _ _ |a 10.1023/A:1015709214016
|g Vol. 42, p. 465 - 492
|p 465 - 492
|q 42<465 - 492
|0 PERI:(DE-600)1475524-5
|t Journal of atmospheric chemistry
|v 42
|y 2002
|x 0167-7764
909 C O |o oai:juser.fz-juelich.de:34365
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|b Environment (Umwelt)
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914 1 _ |y 2002
915 _ _ |0 StatID:(DE-HGF)0010
|a JCR/ISI refereed
920 1 _ |k ICG-II
|l Troposphäre
|d 31.12.2006
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981 _ _ |a I:(DE-Juel1)ICE-3-20101013
981 _ _ |a I:(DE-Juel1)IEK-8-20101013


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