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041 _ _ |a eng
082 _ _ |a 550
084 _ _ |2 WoS
|a Environmental Sciences
084 _ _ |2 WoS
|a Meteorology & Atmospheric Sciences
100 1 _ |a Mannschreck, K.
|b 0
|u FZJ
|0 P:(DE-Juel1)VDB1007
245 _ _ |a Evaluation of the emission inventory by comparisons of modelled and measured emission ratios of individual HCs, CO, and NOx
260 _ _ |a Amsterdam [u.a.]
|b Elsevier Science
|c 2002
300 _ _ |a 81 - 94
336 7 _ |a Journal Article
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336 7 _ |a Journal Article
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336 7 _ |a article
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440 _ 0 |a Atmospheric Environment
|x 1352-2310
|0 697
|v 36
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a Air quality models require emission inventories of individual compounds with high temporal and spatial resolution. These emission inventories are calculated by complex emission models. To evaluate these models, emission ratios of non-methane hydrocarbons (HCs, containing only H- and C-atoms), CO and NOx of the city of Augsburg were determined during two field campaigns in March and October 1998. The measured emission ratios have been compared with emission ratios calculated by an emission model at two accuracy levels.Only C-2-C-10 HCs were measured quantitatively by the applied techniques. C-11-C-13 HCs were measured with losses increasing with the number of C atoms, oxygenated and halogenated volatile organic compounds were not measured at all. The direct comparison could be made only for those HCs whose individual emissions can be specified by the model. They represent 21% of the total predicted volatile organic compound emissions and-according to the model-originate to a large percentage from traffic-related emission. The measured HCi/HCsum emission ratios (HCsum:=Sigma(HCi) for C-2-C-10-HCs and HCi:=mixing ratio of an individual hydrocarbon) for these compounds agreed within 30% for most compounds. The HCi/HCsum emission ratios measured in Augsburg are very similar to emission ratios from traffic-related sources suggesting that the emission model reflects the traffic emissions quite well. In order to consider all measured HCs for comparison the share of unspecified HCs, which are detectable by the GC system and should therefore be included in the experimental results, was estimated. Taking this into account yields a deviation between modelled and measured monthly mean values of HCi/CO and HCi/NOx of about 40%. The comparison of modelled and measured HCi/CO with HCi/HCsum emission ratios derived from the investigation based on single events confirms this finding: in this case an overestimation by the model of a factor of 1.5-2 was found. Since modelled and measured NOx and CO emissions agreed well within the uncertainty ranges, these deviations can be attributed to overestimation of HC emissions.
536 _ _ |a Chemie und Dynamik der Geo-Biosphäre
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588 _ _ |a Dataset connected to Web of Science
650 _ 7 |a J
|2 WoSType
653 2 0 |2 Author
|a hydrocarbon measurements
653 2 0 |2 Author
|a anthropogenic emissions
653 2 0 |2 Author
|a source types
653 2 0 |2 Author
|a emission inventory
653 2 0 |2 Author
|a evaluation
700 1 _ |a Klemp, D.
|b 1
|u FZJ
|0 P:(DE-Juel1)16218
700 1 _ |a Kley, D.
|b 2
|u FZJ
|0 P:(DE-Juel1)16204
700 1 _ |a Friedrich, R.
|b 3
|0 P:(DE-HGF)0
700 1 _ |a Kühlwein, J.
|b 4
|0 P:(DE-HGF)0
700 1 _ |a Wickert, B.
|b 5
|0 P:(DE-HGF)0
700 1 _ |a Matuska, P.
|b 6
|0 P:(DE-HGF)0
700 1 _ |a Habram, M.
|b 7
|0 P:(DE-HGF)0
700 1 _ |a Slemr, E. C.
|b 8
|0 P:(DE-HGF)0
773 _ _ |g Vol. 36, p. 81 - 94
|p 81 - 94
|q 36<81 - 94
|0 PERI:(DE-600)1499889-0
|t Atmospheric environment
|v 36
|y 2002
|x 1352-2310
909 C O |o oai:juser.fz-juelich.de:34367
|p VDB
913 1 _ |k U01
|v Chemie und Dynamik der Geo-Biosphäre
|l Chemie und Dynamik der Geo-Biosphäre
|b Environment (Umwelt)
|0 G:(DE-Juel1)FUEK257
|x 0
914 1 _ |y 2002
915 _ _ |0 StatID:(DE-HGF)0010
|a JCR/ISI refereed
920 1 _ |k ICG-II
|l Troposphäre
|d 31.12.2006
|g ICG
|0 I:(DE-Juel1)VDB48
|x 0
970 _ _ |a VDB:(DE-Juel1)4262
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980 _ _ |a journal
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980 _ _ |a UNRESTRICTED
981 _ _ |a I:(DE-Juel1)ICE-3-20101013
981 _ _ |a I:(DE-Juel1)IEK-8-20101013


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