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@ARTICLE{Ehhalt:34379,
author = {Ehhalt, D. H. and Rohrer, F. and Schauffler, S. and
Pollock, W.},
title = {{T}ritiated water vapor in the stratosphere : vertical
profiles and residence time},
journal = {Journal of Geophysical Research},
volume = {107},
issn = {0148-0227},
address = {Washington, DC},
publisher = {Union},
reportid = {PreJuSER-34379},
pages = {D24},
year = {2002},
note = {Record converted from VDB: 12.11.2012},
abstract = {[1] The historic and partly unpublished measurements of the
tritium content in stratospheric water vapor made at the
National Center for Atmospheric Research between 1975 and
1983 are reanalyzed. The resulting vertical profiles of the
T content, mainly at 32degreesN latitude, show little
variation with altitude above 20 km but a strong decay with
time. This decay is a consequence of the large T injections
into the stratosphere by the atmospheric tests of high-yield
thermonuclear devices prior to 1963 and seems to proceed
with a single e-fold time of 5.12 years. Correcting for the
radioactive decay of HTO within the stratosphere and for a
temporal increase in stratospheric H2O, we obtain a decay
time for stratospheric HTO of 7.7 +/- 2.0 years. This decay
time, which is solely due to the transport of HTO into the
troposphere, is much longer than the age of stratospheric
air at these altitudes or the accepted values for
stratospheric residence times. The differences are discussed
and resolved by interpreting the HTO decay time as the
Eigentime of the longest-lived mode of the stratospheric
transport equations. This Eigentime should provide a useful
constraint in modeling stratospheric transport.},
keywords = {J (WoSType)},
cin = {ICG-II},
ddc = {550},
cid = {I:(DE-Juel1)VDB48},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000181253700007},
doi = {10.1029/2001JD001343},
url = {https://juser.fz-juelich.de/record/34379},
}