001     34882
005     20240712100816.0
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037 _ _ |a PreJuSER-34882
041 _ _ |a eng
082 _ _ |a 550
084 _ _ |2 WoS
|a Meteorology & Atmospheric Sciences
100 1 _ |a Röckmann, T.
|0 P:(DE-HGF)0
|b 0
245 _ _ |a The impact of anthropogenic chlorine emissions, stratospheric ozone change and chemical feedbacks on stratospheric water
260 _ _ |a Katlenburg-Lindau
|b EGU
|c 2004
300 _ _ |a 693 -699
336 7 _ |a Journal Article
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440 _ 0 |a Atmospheric Chemistry and Physics
|x 1680-7316
|0 9601
|v 4
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a Mixing ratios of water (H2O) in the stratosphere appear to increase due to increased input of H2O and methane from the troposphere and due to intensified oxidation of CH4 in the stratosphere, but many of the underlying mechanisms are not yet understood. Here we identify and quantify three chemical mechanisms which must have led to more efficient oxidation of CH4 in the stratosphere over the past several decades: 1) The increase in stratospheric chlorine levels due to anthropogenic CFC emissions, 2) the thinning of the stratospheric ozone column and 3) enhanced OH levels in the stratosphere due to increasing H2O levels themselves. In combination with the increase in tropospheric CH4 mixing ratios and with solar cycle related variations of upper stratospheric ozone, these effects can explain about 50% of the additional conversion of CH4 to H2O as observed throughout the stratosphere. The relative contributions from the individual processes have varied over the past decades.
536 _ _ |a Chemie und Dynamik der Geo-Biosphäre
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588 _ _ |a Dataset connected to Web of Science
650 _ 7 |a J
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700 1 _ |a Grooß, J. U.
|0 P:(DE-Juel1)129122
|b 1
|u FZJ
700 1 _ |a Müller, R.
|0 P:(DE-Juel1)129138
|b 2
|u FZJ
773 _ _ |g Vol. 4, p. 693 -699
|p 693 -699
|q 4<693 -699
|0 PERI:(DE-600)2069847-1
|t Atmospheric chemistry and physics
|v 4
|y 2004
|x 1680-7316
856 4 _ |u https://juser.fz-juelich.de/record/34882/files/R%C3%B6ckmann_2004.Theimpact.pdf
|y OpenAccess
909 C O |o oai:juser.fz-juelich.de:34882
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|v Chemie und Dynamik der Geo-Biosphäre
|l Chemie und Dynamik der Geo-Biosphäre
|b Environment (Umwelt)
|0 G:(DE-Juel1)FUEK257
|x 0
914 1 _ |y 2004
915 _ _ |0 StatID:(DE-HGF)0010
|a JCR/ISI refereed
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|0 StatID:(DE-HGF)0510
|a OpenAccess
920 1 _ |k ICG-I
|l Stratosphäre
|d 31.12.2006
|g ICG
|0 I:(DE-Juel1)VDB47
|x 0
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981 _ _ |a I:(DE-Juel1)IEK-7-20101013


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