TY - JOUR AU - Pavarini, E. AU - Koch, E. AU - Lichtenstein, A. I. TI - Mechanism for Orbital Ordering in KCuF3 JO - Physical review letters VL - 101 SN - 0031-9007 CY - College Park, Md. PB - APS M1 - PreJuSER-3491 SP - 266405 PY - 2008 N1 - Record converted from VDB: 12.11.2012 AB - The Mott insulating perovskite KCuF3 is considered the archetype of an orbitally ordered system. By using the local-density approximation+dynamical mean-field theory method, we investigate the mechanism for orbital ordering in this material. We show that the purely electronic Kugel-Khomskii superexchange mechanism alone leads to a remarkably large transition temperature of T-KK similar to 350 K. However, orbital order is experimentally believed to persist to at least 800 K. Thus, Jahn-Teller distortions are essential for stabilizing orbital order at such high temperatures. KW - J (WoSType) LB - PUB:(DE-HGF)16 UR - <Go to ISI:>//WOS:000262247100057 DO - DOI:10.1103/PhysRevLett.101.266405 UR - https://juser.fz-juelich.de/record/3491 ER -