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000037703 0247_ $$2DOI$$a10.1016/j.susc.2004.03.038
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000037703 084__ $$2WoS$$aChemistry, Physical
000037703 084__ $$2WoS$$aPhysics, Condensed Matter
000037703 1001_ $$0P:(DE-Juel1)VDB5414$$aIbach, H.$$b0$$uFZJ
000037703 245__ $$aThe relation between the strain-dependence of the heat of adsorption and the coverage dependence of the adsorbate induced surface stress
000037703 260__ $$aAmsterdam$$bElsevier$$c2004
000037703 300__ $$a71 - 77
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000037703 440_0 $$05673$$aSurface Science$$v556$$x0039-6028
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000037703 520__ $$aA Maxwell-relation exists between the strain dependence of the chemical potential of an adsorbate and the coverage dependence of the surface stress induced by the same adsorbate. To a good approximation the strain dependence of the chemical potential is equal to the strain dependence of the heat of adsorption. Recent studies on the heat of adsorption of CO on strained Pt(1 1 1) films are discussed in this context and the results are compared to the likewise measured CO-induced surface stress on Pt(1 1 1). It is shown, that the variation of the heat of adsorption with strain depends significantly on the coverage with CO. With reference to the available data on adsorbate induced surface stresses general arguments are presented concerning the sign of the shift in the heat of adsorption with strain and on the general trends in the coverage dependence of the effect. (C) 2004 Published by Elsevier B.V.
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000037703 65320 $$2Author$$aadsorption isotherms
000037703 65320 $$2Author$$achemisorption
000037703 65320 $$2Author$$acatalysis
000037703 65320 $$2Author$$asurface stress
000037703 65320 $$2Author$$aequilibrium thermodynamics and statistical mechanics
000037703 773__ $$0PERI:(DE-600)1479030-0$$a10.1016/j.susc.2004.03.038$$gVol. 556, p. 71 - 77$$p71 - 77$$q556<71 - 77$$tSurface science$$v556$$x0039-6028$$y2004
000037703 8567_ $$uhttp://dx.doi.org/10.1016/j.susc.2004.03.038
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000037703 915__ $$0StatID:(DE-HGF)0010$$aJCR/ISI refereed
000037703 9201_ $$0I:(DE-Juel1)VDB43$$d31.12.2006$$gISG$$kISG-3$$lInstitut für Grenzflächen und Vakuumtechnologien$$x0
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