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@ARTICLE{Giesen:3827,
      author       = {Giesen, M. and Beltramo, G. L. and Dieluweit, S. and
                      Müller, J. and Ibach, H. and Santos, E. and Schmickler, W.},
      title        = {{T}he thermodynamics of electrochemical annealing},
      journal      = {Surface science},
      volume       = {595},
      issn         = {0039-6028},
      address      = {Amsterdam},
      publisher    = {Elsevier},
      reportid     = {PreJuSER-3827},
      year         = {2005},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {We show that on solid electrodes held at constant potential
                      in an electrolyte all defect formation energies and
                      activation energies for surface transport become potential
                      dependent. The rapid smoothening of rough metal electrodes
                      for (mostly) positive electrode potentials ("electrochemical
                      annealing") is therefore the consequence of the specific
                      thermodynamic boundary condition of constant electrode
                      potential. The potential dependence can be related to the
                      surface charge density and the dipole moments of the
                      defects. With dipole moments calculated by ab initio methods
                      the theory is applied to experimental data on
                      two-dimensional Ostwald ripening on Au(1 00) electrodes. The
                      theory is further discussed in the context of other
                      experiments. (c) 2005 Elsevier B.V. All rights reserved.},
      keywords     = {J (WoSType)},
      cin          = {IBN-4},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB802},
      pnm          = {Kondensierte Materie},
      pid          = {G:(DE-Juel1)FUEK414},
      shelfmark    = {Chemistry, Physical / Physics, Condensed Matter},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000233315900016},
      doi          = {10.1016/j.susc.2005.07.040},
      url          = {https://juser.fz-juelich.de/record/3827},
}