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000003828 0247_ $$2DOI$$a10.1016/j.susc.2009.01.006
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000003828 084__ $$2WoS$$aChemistry, Physical
000003828 084__ $$2WoS$$aPhysics, Condensed Matter
000003828 1001_ $$0P:(DE-Juel1)VDB45595$$aMoiseeva, M.$$b0$$uFZJ
000003828 245__ $$aReconstruction on Au(001) Vicinal Surfaces in UHV and in Sulfuric Acid Solution
000003828 260__ $$aAmsterdam$$bElsevier$$c2009
000003828 300__ $$a670 - 675
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000003828 500__ $$aWe acknowledge the skillful sample preparation by U. Linke (www.icryst.com). The work was supported by Deutsche Forschungsgemeinschaft and Fonds der Chemischen Industrie. One of us (H.I.) furthermore acknowledges enlightening discussion with Volker Blum, Fritz-Haber Institute, Berlin, regarding recent progress in total energy calculations on systems with large reconstruction unit cells.
000003828 520__ $$aUsing scanning tunneling microscopy we have studied the reconstruction on Au(1 1 n) surfaces in ultra-high vacuum and in electrolyte. Similar to the well-known (5 x 20) quasi-"hex" reconstruction on Au(0 0 1), the reconstruction consists of parallel reconstruction lines along the steps indicative of a higher atom density in the first Au layer. In contrast to nominally flat Au(0 0 1) where the reconstruction period is 1.44 nm, we find considerably larger reconstruction periods (1.8-1.96 nm) on incidentally flatter regions of nominal Au(1 1 9), Au(1 1 11), and Au(1 1 17) surfaces. The enlarged reconstruction period is attributed to the stress field on stepped surfaces. In agreement with previous studies we find a reconstruction free zone at the step edges. (C) 2009 Elsevier B.V. All rights reserved.
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000003828 65320 $$2Author$$aGold
000003828 65320 $$2Author$$aVicinal single crystal surfaces
000003828 65320 $$2Author$$aMetal-electrolyte interfaces
000003828 65320 $$2Author$$aMetallic surfaces
000003828 65320 $$2Author$$aSurface relaxation and reconstruction
000003828 7001_ $$0P:(DE-Juel1)VDB66689$$aPichardo-Pedrero, E.$$b1$$uFZJ
000003828 7001_ $$0P:(DE-Juel1)128800$$aBeltramo, G. L.$$b2$$uFZJ
000003828 7001_ $$0P:(DE-Juel1)VDB5414$$aIbach, H.$$b3$$uFZJ
000003828 7001_ $$0P:(DE-Juel1)4744$$aGiesen, M.$$b4$$uFZJ
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000003828 8567_ $$uhttp://dx.doi.org/10.1016/j.susc.2009.01.006
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