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@ARTICLE{Plenge:39737,
      author       = {Plenge, J. and Flesch, R. and Kühl, S. and Vogel, B. and
                      Müller, R. and Stroh, F. and Rühl, E.},
      title        = {{U}ltraviolet {P}hotolysis of the {C}l{O} {D}imer},
      journal      = {The journal of physical chemistry / A},
      volume       = {108},
      issn         = {1089-5639},
      address      = {Washington, DC},
      publisher    = {Soc.},
      reportid     = {PreJuSER-39737},
      pages        = {4859 - 4863},
      year         = {2004},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {Photodissociation of the ClO dimer (ClOOCl) is studied in
                      the ultraviolet regime (250 and 308 nm) under collision-free
                      conditions. The primary photolysis products are probed by
                      photoionization mass spectrometry. At both photolysis
                      wavelengths, exclusively the formation of 2Cl + O-2 is
                      observed, corresponding to a primary quantum yield gamma(Cl)
                      near unity. Considering the error limit of the experimental
                      results one obtains gamma(Cl) greater than or equal to 0.98
                      at 250 nm and gamma(Cl) greater than or equal to 0.90 at 308
                      nm, respectively. At both photolysis wavelengths the pathway
                      yielding ClO is not observed, corresponding to gamma(ClO)
                      less than or equal to 0.02 at 250 nm and gamma(ClO) less
                      than or equal to 0.10 at 308 nm. Sensitivity studies of
                      these results with respect to ozone depletion in the
                      stratosphere regarding photochemically induced ozone loss
                      are discussed using model simulations. These simulations
                      suggest that a change of gamma(Cl) from 1.0 to 0.9 leads to
                      a reduction of polar ozone loss of similar $to5\%.$},
      keywords     = {J (WoSType)},
      cin          = {ICG-I},
      ddc          = {530},
      cid          = {I:(DE-Juel1)VDB47},
      pnm          = {Chemie und Dynamik der Geo-Biosphäre},
      pid          = {G:(DE-Juel1)FUEK257},
      shelfmark    = {Chemistry, Physical / Physics, Atomic, Molecular $\&$
                      Chemical},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000221700100006},
      doi          = {10.1021/jp049690+},
      url          = {https://juser.fz-juelich.de/record/39737},
}