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@ARTICLE{Wandlowski:40430,
      author       = {Wandlowski, T. and Wang, J. X. and Ocko, B. M.},
      title        = {{A}dsorption of bromide at the {A}g(100) electrode surface},
      journal      = {Journal of electroanalytical chemistry},
      volume       = {500},
      issn         = {0022-0728},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {PreJuSER-40430},
      pages        = {418},
      year         = {2001},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The adsorption and phase formation of bromide on Ag(100)
                      has been studied by chronocoulometry and surface X-ray
                      scattering (SXS). With increasing electrode potential,
                      bromide undergoes a phase transition from a lattice gas to
                      an ordered c(2 x 2) structure (theta = 0.5). The degree of
                      lateral disorder was estimated by comparing the SXS- and the
                      electrochemical measurements. Based on chronocoulometric
                      experiments, a thermodynamic analysis of charge density data
                      was performed to describe the bromide adsorption at the
                      Ag(100) electrode. The Gibbs surfaces excess,
                      electrosorption valencies, Esin-Markov coefficients, and the
                      Gibbs energy of adsorption, lateral interaction energies as
                      well as surface dipole moments have been estimated. The
                      experimental theta versus E- isotherms are modeled employing
                      (i) a quasi-chemical approximation as well as (ii) the
                      results of a recent Monte Carlo simulation. An attempt is
                      made to discuss the structure data and thermodynamic
                      quantities of bromide adsorption on Ag(100) on the basis of
                      the Grahame-Parsons model of the Helmholtz layer. (C) 2001
                      Elsevier Science B.V. All rights reserved.},
      keywords     = {J (WoSType)},
      cin          = {ISG-3 / IFF-IMF},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB43 / I:(DE-Juel1)VDB37},
      pnm          = {Struktur und Dynamik von Grenzflächen},
      pid          = {G:(DE-Juel1)FUEK60},
      shelfmark    = {Chemistry, Analytical / Electrochemistry},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000168192000046},
      doi          = {10.1016/S0022-0728(00)00380-6},
      url          = {https://juser.fz-juelich.de/record/40430},
}