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@ARTICLE{Bhakta:41145,
author = {Bhakta, R. and Thomas, R. and Hipler, F. and Bettinger, H.
and Müller, J. and Ehrhart, P. and Devi, A.},
title = {{MOCVD} of {T}i{O}2 thin films and studies on the nature of
molecular mechanisms involved in the decomposition of
[{T}i({OP}ri)2(tbaoac)2]},
journal = {Journal of materials chemistry},
volume = {14},
issn = {0959-9428},
address = {London},
publisher = {ChemSoc},
reportid = {PreJuSER-41145},
pages = {3231 - 3238},
year = {2004},
note = {Record converted from VDB: 12.11.2012},
abstract = {A tailored precursor namely
bis(isopropoxy)bis(tert-butylacetoacetato)titanium
[Ti(OPri)(2)(tbaoac)(2)] was developed which showed good
promise for depositing TiO2 thin films at reduced substrate
temperatures compared to [Ti(OPri)(2)(thd)(2)]. Uniform
films with high growth rates (similar to10 nm min(-1)) and
lower surface roughness (<2 nm) were obtained on SiOx/Si and
Pt/ZrOx/SiOx/Si substrates. Electrical properties of the
films on Si substrates were studied and lowest equivalent
oxide thickness (EOT) was around 2 nm and anatase phase had
a dielectric constant around 40. A study on the thermolysis
behaviour of [Ti(OPri)(2)(tbaoac)(2)] was carried out using
matrix-isolation FTIR spectroscopy, to understand the
mechanistic details of its thermal decomposition. It was
found that the decomposition takes place by the formation of
ketene intermediates.},
keywords = {J (WoSType)},
cin = {IFF-IEM / CNI},
ddc = {540},
cid = {I:(DE-Juel1)VDB321 / I:(DE-Juel1)VDB381},
pnm = {Materialien, Prozesse und Bauelemente für die Mikro- und
Nanoelektronik},
pid = {G:(DE-Juel1)FUEK252},
shelfmark = {Chemistry, Physical / Materials Science, Multidisciplinary},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000224735700021},
doi = {10.1039/b405963h},
url = {https://juser.fz-juelich.de/record/41145},
}