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@ARTICLE{Anttila:42749,
author = {Anttila, T. and Kerminen, V.-M. and Kulmala, M. and
Laaksonen, A. and O'Dowd, C.},
title = {{M}odelling the formation of organic particles in the
atmosphere},
journal = {Atmospheric chemistry and physics},
volume = {4},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-42749},
pages = {1071 - 1083},
year = {2004},
note = {Record converted from VDB: 12.11.2012},
abstract = {Particle formation resulting from activation of inorganic
stable clusters by a supersaturated organic vapour was
investigated using a numerical model. The applied aerosol
dynamic model included a detailed description of the
activation process along with a treatment of the appropriate
aerosol and gas-phase processes. The obtained results
suggest that both gaseous sulphuric acid and organic vapours
contribute to organic particle formation in continental
background areas. The initial growth of freshly-nucleated
clusters is driven mainly by condensation of gaseous
sulphuric acid and by a lesser extent self-coagulation.
After the clusters have reached sizes of around 2 nm in
diameter, low-volatile organic vapours start to condense
spontaneously into the clusters, thereby accelerating their
growth to detectable sizes. A shortage of gaseous sulphuric
acid or organic vapours limit, or suppress altogether, the
particle formation, since freshly-nucleated clusters are
rapidly coagulated away by pre-existing particles. The
obtained modelling results were applied to explaining the
observed seasonal cycle in the number of aerosol formation
events in a continental forest site.},
keywords = {J (WoSType)},
cin = {ICG-II},
ddc = {550},
cid = {I:(DE-Juel1)VDB48},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000222473800003},
url = {https://juser.fz-juelich.de/record/42749},
}