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@ARTICLE{Lustfeld:42902,
      author       = {Lustfeld, H. and Pohlmeier, A.},
      title        = {{E}lectric potential and reaction rates at charged surfaces
                      in asymmetric electrolytes : an analytical approach},
      journal      = {Journal of colloid and interface science},
      volume       = {239},
      issn         = {0021-9797},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier},
      reportid     = {PreJuSER-42902},
      pages        = {113 - 125},
      year         = {2001},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The electric potential and reaction rates of ions hitting
                      the chemically active surfaces of microcrystals in an
                      asymmetric electrolyte are computed analytically. Following
                      ideas of Debye we start by solving the Poisson-Boltzmann
                      equations and by determining the electric potential of the
                      transport equations. We find distinct deviations when
                      comparing our result with the Gouy-Chapman formula. In a
                      simple model approximating a situation in which lead and
                      hydrogen ions can react at goethite surfaces we compute
                      analytically the currents of ions diffusing to the surfaces
                      of microcrystals where they undergo a chemical reaction. We
                      compute the reaction rates that can be controlled either by
                      chemical reactions at the surface of the microcrystals or by
                      diffusional transport. For realistic parameters of our model
                      we find that the diffusional transport is the rate
                      determining step. Copyright 2001 Academic Press.},
      keywords     = {J (WoSType)},
      cin          = {IFF-TH-I / ICG-IV},
      ddc          = {540},
      cid          = {I:(DE-Juel1)VDB30 / I:(DE-Juel1)VDB50},
      pnm          = {Elektronische Struktur von Festkörpern, Oberflächen und
                      Schichtsystemen / Stoffströme von Schwermetallen und
                      organischen Substanzen in der Umwelt},
      pid          = {G:(DE-Juel1)FUEK52 / G:(DE-Juel1)FUEK83},
      shelfmark    = {Chemistry, Physical},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:11397055},
      UT           = {WOS:000169533100015},
      doi          = {10.1006/jcis.2001.7486},
      url          = {https://juser.fz-juelich.de/record/42902},
}