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@ARTICLE{Spirig:44372,
author = {Spirig, C. and Neftel, A. and Ammann, C. and Dommen, G. Di.
and Grabmer, W. and Thielmann, A. and Schaub, A. and
Beauchamp, J. and Wisthaler, A. and Hansel, A.},
title = {{E}ddy covariance flux measurements of biogenic {VOC}s
during {ECHO} 2003 using proton transfer reaction mass
spectrometry},
journal = {Atmospheric chemistry and physics},
volume = {5},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-44372},
pages = {465 - 481},
year = {2005},
note = {Record converted from VDB: 12.11.2012},
abstract = {Within the framework of the AFO 2000 project ECHO, two
PTR-MS instruments were operated in combination with sonic
anemometers to determine biogenic VOC fluxes from a mixed
deciduous forest site in North-Western Germany. The
measurement site was characterised by a forest of
inhomogeneous composition, complex canopy structure, limited
extension in certain wind directions and frequent calm wind
conditions during night time. The eddy covariance (EC)
technique was applied since it represents the most direct
flux measurement approach on the canopy scale and is,
therefore, least susceptible to these non-ideal conditions.
A specific flux calculation method was used to account for
the sequential multi-component PTR-MS measurements and
allowing an individual delay time adjustment as well as a
rigorous quality control based on cospectral analysis. The
validated flux results are consistent with light and
temperature dependent emissions of isoprene and monoterpenes
from this forest, with average daytime emissions of 0.94 and
0.3 mug m(-2) s(-1), respectively. Emissions of methanol
reached on average 0.087 mug m(-2) s(-1) during daytime, but
fluxes were too small to be detected during night time.
Upward fluxes of the isoprene oxidation products methyl
vinyl ketone (MVK) and methacrolein (MACR) were also found,
being two orders of magnitude lower than those of isoprene.
Calculations with an analytical footprint model indicate
that the observed isoprene fluxes correlate with the
fraction of oaks within the footprints of the flux
measurement.},
keywords = {J (WoSType)},
cin = {ICG-II},
ddc = {550},
cid = {I:(DE-Juel1)VDB48},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000226995100001},
url = {https://juser.fz-juelich.de/record/44372},
}