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@ARTICLE{Voigt:45971,
author = {Voigt, C. and Schlager, H. and Luo, B. and Dörnbrack, A.
and Roiger, A. and Stock, P. and Curtius, J. and Vössing,
H. and Borrmann, S. and Davies, S. and Konopka, Paul and
Schiller, C. and Shur, G. and Peter, T.},
title = {{N}itric acid trihydrate ({NAT}) formation at low {NAT}
supersaturations in {P}olar {S}tratospheric {C}louds
({PSC}s)},
journal = {Atmospheric chemistry and physics},
volume = {5},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-45971},
pages = {1371-1380},
year = {2005},
note = {Record converted from VDB: 12.11.2012},
abstract = {A PSC was detected on 6 February 2003 in the Arctic
stratosphere by in-situ measurements onboard the
high-altitude research aircraft Geophysica. Low number
densities (similar to 10(-4) cm(-3)) of small nitric acid
(HNO3) containing particles (d< 6 mu m) were observed at
altitudes between 18 and 20 km. Provided the temperatures
remain below the NAT equilibrium temperature TNAT, these NAT
particles have the potential to grow further and to remove
HNO3 from the stratosphere, thereby enhancing polar ozone
loss. Interestingly, the NAT particles formed in less than a
day at temperatures just slightly below T-NAT ( T> T-NAT-
3.1 K). This unique measurement of PSC formation at
extremely low NAT saturation ratios (S-NAT less than or
similar to 10) constrains current NAT nucleation theories.
We suggest, that the NAT particles have formed
heterogeneously, but for certain not on ice. Conversely,
meteoritic particles may be favorable candidates for
triggering NAT nucleation at the observed low number
densities.},
keywords = {J (WoSType)},
cin = {ICG-I},
ddc = {550},
cid = {I:(DE-Juel1)VDB47},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000229615500002},
url = {https://juser.fz-juelich.de/record/45971},
}