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@ARTICLE{Postnikov:46132,
author = {Postnikov, A. V. and Pagès, O. and Hugel, J. A.},
title = {{L}attice dynamics of the mixed semiconductors ({B}e,
{Z}n){S}e from first-principles calculations},
journal = {Physical review / B},
volume = {71},
number = {11},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {PreJuSER-46132},
pages = {115206},
year = {2005},
note = {Record converted from VDB: 12.11.2012},
abstract = {Vibration properties of Zn1-xBexSe, a mixed II-VI
semiconductor characterized by a high contrast in elastic
properties of its pure constituents ZnSe and BeSe, are
simulated by first-principles calculations of electronic
structure, lattice relaxation, and frozen phonons. The
calculations within the local density approximation have
been done with the SIESTA method, using norm-conserving
pseudopotentials and localized basis functions; the
benchmark calculations for pure end systems were, moreover,
done also by the all-electron WIEN2k code. An immediate
motivation for the study was to analyze, at the microscopic
level, the appearance of anomalous phonon modes detected
early in Raman spectra in the intermediate region
$(20\%-80\%)$ of ZnBe concentration. This was discussed
early on the basis of a percolation phenomenon-i.e., the
result of the formation of wall-to-wall -Be-Se- chains
throughout the crystal. The presence of such chains was
explicitly allowed in our simulation and indeed brought
about a softening and splitting off of particular modes, in
accordance with experimental observation, due to a relative
elongation of Be-Se bonds along the chain as compared to
those involving isolated Be atoms. The variation of force
constants with interatomic distances shows common trends in
relative independence of the short-range order.},
keywords = {J (WoSType)},
cin = {IFF-TH-I},
ddc = {530},
cid = {I:(DE-Juel1)VDB30},
pnm = {Kondensierte Materie},
pid = {G:(DE-Juel1)FUEK242},
shelfmark = {Physics, Condensed Matter},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000228065500065},
doi = {10.1103/PhysRevB.71.115206},
url = {https://juser.fz-juelich.de/record/46132},
}