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@ARTICLE{Witthuhn:46549,
author = {Witthuhn, B. and Pernyeszi, S. K. and Klauth, P. and
Vereecken, H. and Klumpp, E.},
title = {{S}orption study of 2,4-dichlorophenol on organoclays
constructed for soil bioremediation},
journal = {Colloids and surfaces / A},
volume = {265},
issn = {0927-7757},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PreJuSER-46549},
pages = {81 - 87},
year = {2005},
note = {Record converted from VDB: 12.11.2012},
abstract = {The role of the type and amount of cationic surfactant in
the sorption behaviour of partially modified clays was
studied and the applicability of a partially modified
organoclay for bioremediation was demonstrated. Partially
modified surfactant/clay complexes ("organoclays") were
prepared from Na-montmorillonite by using
monoalkyl-(dodecyltrimethylammonium and
octadecyltrimethylammonium) and dialkylammonium
(didodecyldimethylammonium and dioctadecyldimethylammonium)
bromides. The degree of modification was varied between 35
and $89\%$ of the cation exchange capacity of
montmorillonite (MM). The sorption of 2,4-dichlorophenol
(DCP) on organoclays was studied by using the batch
technique. The intercalation of DCP into the interlayers of
organo-MM was detected by X-ray diffraction. The adsorption
isotherms found were non-linear indicating that the sorption
is not only based on a simple partition mechanism. The
adsorption coefficients K-d calculated from the initial
isotherm slope turned out to be exponential with the organic
carbon content of organo-MM (integral(oc)) In particular,
dialkylammonium-modified MM revealed outstanding sorption
characteristics for DCP. The comparison of partially
modified organo-MMs with similar integral(oc) and volume
fraction of surfactant indicated that the surfactant
arrangement in the interlayers significantly influences the
DCP adsorption. It-could be assumed that both the kind and
degree of exchanged surfactant play a decisive role in the
adsorption of DCP on the organoclays. By performing
biodegradation experiments in the presence of
dioctadecyldimethylammonium montmorillonite, the complete
biodegradation of DCP was achieved demonstrating the
applicability of partially modified organoclays for
bioremediation. (c) 2005 Elsevier B.V. All rights reserved.},
keywords = {J (WoSType)},
cin = {ICG-IV},
ddc = {540},
cid = {I:(DE-Juel1)VDB50},
pnm = {Chemie und Dynamik der Geo-Biosphäre},
pid = {G:(DE-Juel1)FUEK257},
shelfmark = {Chemistry, Physical},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000231379100010},
doi = {10.1016/j.colsurfa.2004.11.049},
url = {https://juser.fz-juelich.de/record/46549},
}