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@ARTICLE{Brown:4663,
      author       = {Brown, S.S. and Dubé, W. P. and Fuchs, H. and Ryerson,
                      T.B. and Wollny, A.G. and Brock, C.A. and Bahreini, R. and
                      Middlebrook, A.M. and Neuman, J.A. and Atlas, E. and
                      Roberts, J.M. and Osthoff, H.D. and Trainer, M. and
                      Fehsenfeld, F.C. and Ravishankara, A.R.},
      title        = {{R}eactive uptake coefficients for {N}2{O}5 determined from
                      aircraft measuremnts during the {S}econd {T}exas {A}ir
                      {Q}uality {S}tudy: {C}omparison to current model
                      parameterizations},
      journal      = {Journal of Geophysical Research},
      volume       = {114},
      issn         = {0148-0227},
      address      = {Washington, DC},
      publisher    = {Union},
      reportid     = {PreJuSER-4663},
      pages        = {1 - 16},
      year         = {2009},
      note         = {This work was supported by the NOAA Atmospheric Chemistry
                      and Climate Program and the Texas Air Quality Study. The
                      authors thank Prakash Bhave for useful discussions regarding
                      uptake coefficient parameterizations. The authors also thank
                      the crew of the NOAA P-3 for their dedication and
                      professionalism.},
      abstract     = {This paper presents determinations of reactive uptake
                      coefficients for N2O5, gamma( N2O5), on aerosols from
                      nighttime aircraft measurements of ozone, nitrogen oxides,
                      and aerosol surface area on the NOAA P-3 during Second Texas
                      Air Quality Study (TexAQS II). Determinations based on both
                      the steady state approximation for NO3 and N2O5 and a plume
                      modeling approach yielded gamma(N2O5) substantially smaller
                      than current parameterizations used for atmospheric modeling
                      and generally in the range 0.5-6 x 10(-3). Dependence of
                      gamma(N2O5) on variables such as relative humidity and
                      aerosol composition was not apparent in the determinations,
                      although there was considerable scatter in the data.
                      Determinations were also inconsistent with current
                      parameterizations of the rate coefficient for homogenous
                      hydrolysis of N2O5 by water vapor, which may be as much as a
                      factor of 10 too large. Nocturnal halogen activation via
                      conversion of N2O5 to ClNO2 on chloride aerosol was not
                      determinable from these data, although limits based on
                      laboratory parameterizations and maximum nonrefractory
                      aerosol chloride content showed that this chemistry could
                      have been comparable to direct production of HNO3 in some
                      cases.},
      keywords     = {J (WoSType)},
      cin          = {ICG-2},
      ddc          = {550},
      cid          = {I:(DE-Juel1)VDB791},
      pnm          = {Atmosphäre und Klima},
      pid          = {G:(DE-Juel1)FUEK406},
      shelfmark    = {Meteorology $\&$ Atmospheric Sciences},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000266742600006},
      doi          = {10.1029/2008JD011679},
      url          = {https://juser.fz-juelich.de/record/4663},
}