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@ARTICLE{Plieth:46693,
author = {Plieth, W. and Lorenz, W. J. and Staikov, G.},
title = {{B}ond {E}nergies in {A}lloys {D}etermined from
{U}nderpotential {D}eposition {P}otentials},
journal = {Journal of solid state electrochemistry},
volume = {8},
issn = {1432-8488},
address = {Berlin},
publisher = {Springer},
reportid = {PreJuSER-46693},
pages = {941 - 946},
year = {2004},
note = {Record converted from VDB: 12.11.2012},
abstract = {A procedure is presented to determine bond energies between
the metal (Me) and substrate (S) components of binary alloys
from characteristic underpotential deposition (UPD)
potentials. The bond energy between Me and S atoms is one of
the factors governing the deposition kinetics and structure
of Me-S alloy deposits. The proposed procedure is based on
the determination of the UPD potential for formation of a
condensed two-dimensional (2D) phase of the less noble metal
Me (the UPD metal) on the more noble metal S (the
substrate). Making reasonable approximations, the
sublimation enthalpy of the condensed 2D Me phase is
obtained from the corresponding formation underpotential.
From this sublimation enthalpy the bond energy of an atom of
the UPD metal in a kink site position of the 2D Me phase is
calculated. This value is used to calculate the bond energy
(phi(Me-S)) between an Me atom and an S atom. The method is
demonstrated using experimental data obtained in selected
electrochemical UPD systems.},
keywords = {J (WoSType)},
cin = {ISG-3},
ddc = {540},
cid = {I:(DE-Juel1)VDB43},
pnm = {Kondensierte Materie},
pid = {G:(DE-Juel1)FUEK242},
shelfmark = {Electrochemistry},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000224836000002},
doi = {10.1007/s10008-004-0513-1},
url = {https://juser.fz-juelich.de/record/46693},
}