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000046780 084__ $$2WoS$$aPhysics, Atomic, Molecular & Chemical
000046780 1001_ $$0P:(DE-HGF)0$$aHofmann, T.$$b0
000046780 245__ $$aIntegral equation theory approach to rodlike polyelectrolytes : counterion condensation
000046780 260__ $$aMelville, NY$$bAmerican Institute of Physics$$c2001
000046780 300__ $$a10181
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000046780 440_0 $$03145$$aJournal of Chemical Physics$$v114$$x0021-9606$$y22
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000046780 520__ $$aWe investigate the structural properties of rigid linear polyelectrolytes in dilute and semidilute solutions using an integral equation theory. The Polymer Reference Interaction Site Model together with the Reference Laria Wu Chandler Closure is solved numerically taking the counterions into account explicitly. The counterions and the polymer chains, modeled as linearly connected, charged hard spheres, interact through an unscreened Coulomb potential. The pair correlation functions between the monomers of different chains, the counterions, and the monomers and counterions, respectively, are calculated for various densities and Bjerrum lengths. Based upon these quantities, the effective potential among the monomers and the counterions, respectively, is extracted. In particular, a critical Bjerrum length is determined, which separates the regime of a repulsive interaction between the counterions from the regime of an attractive interaction transmitted by the polymer chains. (C) 2001 American Institute of Physics.
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000046780 7001_ $$0P:(DE-Juel1)131039$$aWinkler, R. G.$$b1$$uFZJ
000046780 7001_ $$0P:(DE-HGF)0$$aReineker, P.$$b2
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