000046870 001__ 46870 000046870 005__ 20200402205958.0 000046870 0247_ $$2DOI$$a10.1002/1438-5171(200103)2:1<35::AID-SIMO35>3.3.CO;2-C 000046870 0247_ $$2WOS$$aWOS:000174074400006 000046870 037__ $$aPreJuSER-46870 000046870 041__ $$aeng 000046870 082__ $$a570 000046870 084__ $$2WoS$$aBiochemical Research Methods 000046870 084__ $$2WoS$$aBiochemistry & Molecular Biology 000046870 084__ $$2WoS$$aChemistry, Multidisciplinary 000046870 1001_ $$0P:(DE-Juel1)131924$$aGensch, T.$$b0$$uFZJ 000046870 245__ $$aPolarisation sensitive single molecule fluorescence detection with linear polarised excitation light and modulated polarisation direction applied to multichromophoric entities 000046870 260__ $$aBerlin$$bWiley-VCH$$c2001 000046870 300__ $$a35 - 44 000046870 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article 000046870 3367_ $$2DataCite$$aOutput Types/Journal article 000046870 3367_ $$00$$2EndNote$$aJournal Article 000046870 3367_ $$2BibTeX$$aARTICLE 000046870 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000046870 3367_ $$2DRIVER$$aarticle 000046870 440_0 $$06630$$aSingle Molecules$$v2$$x1438-5163 000046870 500__ $$aRecord converted from VDB: 12.11.2012 000046870 520__ $$aRecently, investigations of the fluorescence properties of a multichromophoric dendritic entity at the single molecule level have revealed multiple fluorescence levels, collective off-states, variations of the polarisation, large shifts in the spectral position and changes in the fluorescence decay time (Gensch et al. (1999), Hofkens et al. (2000)). In order to further elucidate the multiple processes taking place in this entity, measurements were done in which the polarisation direction of the linear polarised excitation light was modulated. The detection was sensitive for the s- and p-components of the emitted light. The patterns of modulation and relative intensity in the acquired traces reflect the energy transfer processes occurring in this multichromophoric molecule. In-phase modulation and no modulation are the typical modulation patterns that were observed. Simulations involving several models for energy transfer between the chromophores have been carried out taking into account identical conditions as for the performed measurements. The comparison of the modulation patterns and polarisation histograms to the measured data rules out certain models and refines the photophysical model for the multichromophoric entity. 000046870 536__ $$0G:(DE-Juel1)FUEK95$$2G:(DE-HGF)$$aZelluläre Signalverarbeitung$$c42.20.1$$x0 000046870 588__ $$aDataset connected to Web of Science 000046870 650_7 $$2WoSType$$aJ 000046870 7001_ $$0P:(DE-HGF)0$$aHofkens, J.$$b1 000046870 7001_ $$0P:(DE-HGF)0$$aKoehn, F.$$b2 000046870 7001_ $$0P:(DE-HGF)0$$aVosch, T.$$b3 000046870 7001_ $$0P:(DE-HGF)0$$aHerrmann, A.$$b4 000046870 7001_ $$0P:(DE-HGF)0$$aMuellen, K.$$b5 000046870 7001_ $$0P:(DE-HGF)0$$ade Schryver, F. C.$$b6 000046870 773__ $$0PERI:(DE-600)2011809-0$$a10.1002/1438-5171(200103)2:1<35::AID-SIMO35>3.3.CO;2-C$$gVol. 2, p. 35 - 44$$p35 - 44$$q2<35 - 44$$tSingle molecules$$v2$$x1438-5163$$y2001 000046870 909CO $$ooai:juser.fz-juelich.de:46870$$pVDB 000046870 9131_ $$0G:(DE-Juel1)FUEK95$$bLebenswissenschaften$$k42.20.1$$lBiologische Informationsverarbeitung$$vZelluläre Signalverarbeitung$$x0 000046870 9141_ $$y2001 000046870 915__ $$0StatID:(DE-HGF)0010$$aJCR/ISI refereed 000046870 9201_ $$0I:(DE-Juel1)VDB57$$d31.12.2006$$gIBI$$kIBI-1$$lZelluläre Signalverarbeitung$$x0 000046870 970__ $$aVDB:(DE-Juel1)977 000046870 980__ $$aVDB 000046870 980__ $$aConvertedRecord 000046870 980__ $$ajournal 000046870 980__ $$aI:(DE-Juel1)ICS-4-20110106 000046870 980__ $$aUNRESTRICTED 000046870 981__ $$aI:(DE-Juel1)IBI-1-20200312 000046870 981__ $$aI:(DE-Juel1)ICS-4-20110106