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@ARTICLE{Gensch:46870,
      author       = {Gensch, T. and Hofkens, J. and Koehn, F. and Vosch, T. and
                      Herrmann, A. and Muellen, K. and de Schryver, F. C.},
      title        = {{P}olarisation sensitive single molecule fluorescence
                      detection with linear polarised excitation light and
                      modulated polarisation direction applied to
                      multichromophoric entities},
      journal      = {Single molecules},
      volume       = {2},
      issn         = {1438-5163},
      address      = {Berlin},
      publisher    = {Wiley-VCH},
      reportid     = {PreJuSER-46870},
      pages        = {35 - 44},
      year         = {2001},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {Recently, investigations of the fluorescence properties of
                      a multichromophoric dendritic entity at the single molecule
                      level have revealed multiple fluorescence levels, collective
                      off-states, variations of the polarisation, large shifts in
                      the spectral position and changes in the fluorescence decay
                      time (Gensch et al. (1999), Hofkens et al. (2000)). In order
                      to further elucidate the multiple processes taking place in
                      this entity, measurements were done in which the
                      polarisation direction of the linear polarised excitation
                      light was modulated. The detection was sensitive for the s-
                      and p-components of the emitted light. The patterns of
                      modulation and relative intensity in the acquired traces
                      reflect the energy transfer processes occurring in this
                      multichromophoric molecule. In-phase modulation and no
                      modulation are the typical modulation patterns that were
                      observed. Simulations involving several models for energy
                      transfer between the chromophores have been carried out
                      taking into account identical conditions as for the
                      performed measurements. The comparison of the modulation
                      patterns and polarisation histograms to the measured data
                      rules out certain models and refines the photophysical model
                      for the multichromophoric entity.},
      keywords     = {J (WoSType)},
      cin          = {IBI-1},
      ddc          = {570},
      cid          = {I:(DE-Juel1)VDB57},
      pnm          = {Zelluläre Signalverarbeitung},
      pid          = {G:(DE-Juel1)FUEK95},
      shelfmark    = {Biochemical Research Methods / Biochemistry $\&$ Molecular
                      Biology / Chemistry, Multidisciplinary},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000174074400006},
      doi          = {10.1002/1438-5171(200103)2:1<35::AID-SIMO35>3.3.CO;2-C},
      url          = {https://juser.fz-juelich.de/record/46870},
}