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@ARTICLE{Fry:4703,
      author       = {Fry, J.L. and Kiendler-Scharr, A. and Rollins, A.W. and
                      Wooldridge, P.J. and Brown, S.S. and Fuchs, H. and Dube, W.
                      and Mensah, A. and Dal Maso, M. and Tillmann, R. and Dorn,
                      H.-P. and Brauers, T. and Cohen, R.C.},
      title        = {{O}rganic nitrate and secondary organic aerosol yield from
                      {NO}3 oxidation of ß-pinene evaluated using a gas-phase
                      kinetics/aerosol partitioning model},
      journal      = {Atmospheric chemistry and physics},
      volume       = {9},
      issn         = {1680-7316},
      address      = {Katlenburg-Lindau},
      publisher    = {EGU},
      reportid     = {PreJuSER-4703},
      pages        = {1431 - 1449},
      year         = {2009},
      note         = {The Berkeley authors were supported by NSF ATM-0639847 and
                      NSF ATM-0511829. The authors thank Luke Valin for assistance
                      running WRF/Chem; Klaus Scott for providing California
                      monoterpene emissions estimates; Steve Ball and Bill Simpson
                      for helpful comments on the manuscript; and the entire
                      SAPHIR NO<INF>3</INF> intercomparison campaign team, June
                      2007 at Forschungszentrum Julich, for their support of these
                      experiments. This work was a joint activity of the European
                      Network of Excellence ACCENT ( contract no: GOCE
                      CT-2004-505337) and EUROCHAMP.},
      abstract     = {The yields of organic nitrates and of secondary organic
                      aerosol (SOA) particle formation were measured for the
                      reaction NO3+beta-pinene under dry and humid conditions in
                      the atmosphere simulation chamber SAPHIR at Research Center
                      Julich. These experiments were conducted at low
                      concentrations of NO3 (NO3+N2O5 < 10 ppb) and beta-pinene
                      (peak similar to 15 ppb), with no seed aerosol. SOA
                      formation was observed to be prompt and substantial (similar
                      to $50\%$ mass yield under both dry conditions and at $60\%$
                      RH), and highly correlated with organic nitrate formation.
                      The observed gas/aerosol partitioning of organic nitrates
                      can be simulated using an absorptive partitioning model to
                      derive an estimated vapor pressure of the condensing nitrate
                      species of p(vap) similar to 5x10(-6) Torr (6.67x10(-4) Pa),
                      which constrains speculation about the oxidation mechanism
                      and chemical identity of the organic nitrate. Once formed
                      the SOA in this system continues to evolve, resulting in
                      measurable aerosol volume decrease with time. The
                      observations of high aerosol yield from NOx-dependent
                      oxidation of monoterpenes provide an example of a
                      significant anthropogenic source of SOA from biogenic
                      hydrocarbon precursors. Estimates of the NO3+beta-pinene SOA
                      source strength for California and the globe indicate that
                      NO3 reactions with monoterpenes are likely an important
                      source $(0.5-8\%$ of the global total) of organic aerosol on
                      regional and global scales.},
      keywords     = {J (WoSType)},
      cin          = {ICG-2},
      ddc          = {550},
      cid          = {I:(DE-Juel1)VDB791},
      pnm          = {Atmosphäre und Klima},
      pid          = {G:(DE-Juel1)FUEK406},
      shelfmark    = {Meteorology $\&$ Atmospheric Sciences},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000263642000024},
      url          = {https://juser.fz-juelich.de/record/4703},
}