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@ARTICLE{Riemer:4707,
      author       = {Riemer, N. and Vogel, H. and Anttila, T. and
                      Kiendler-Scharr, A. and Mentel, T. F.},
      title        = {{R}elative importance of organic coatings for the
                      heterogeneous hydrolysis of {N}2{O}5 during summer in
                      {E}urope},
      journal      = {Journal of Geophysical Research},
      volume       = {114},
      issn         = {0148-0227},
      address      = {Washington, DC},
      publisher    = {Union},
      reportid     = {PreJuSER-4707},
      pages        = {D17307},
      year         = {2009},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The heterogeneous reaction probability gamma N2O5 of N2O5
                      depends largely on the aerosol chemical composition. Several
                      recent laboratory studies have shown that the presence of
                      organic coatings on aqueous aerosols can suppress
                      heterogeneous N2O5 hydrolysis. In this study we investigated
                      the relative importance of organic coatings, formed via
                      gas-to-particle conversion on aqueous aerosols, to N2O5
                      hydrolysis on local and regional scales during summer in
                      Europe. We present results of one-dimensional process
                      studies and of regional-scale model simulations for Europe
                      with the comprehensive model system COSMO-ART. To treat N2O5
                      hydrolysis, we used recent results from laboratory studies
                      that quantified gamma N2O5 on the basis of the organic
                      coating thickness. The simulations showed that during any
                      episode the conditions for formation of N2O5 and secondary
                      organic compounds were very variable and depended strongly
                      on the meteorological conditions. In regions of the model
                      domain where both components were built-up, the formation of
                      organic coatings could decrease particulate nitrate
                      concentrations by up to $90\%.$ Where these conditions were
                      not met, the impact of the organic coating was negligible.},
      keywords     = {J (WoSType)},
      cin          = {ICG-2},
      ddc          = {550},
      cid          = {I:(DE-Juel1)VDB791},
      pnm          = {Atmosphäre und Klima},
      pid          = {G:(DE-Juel1)FUEK406},
      shelfmark    = {Meteorology $\&$ Atmospheric Sciences},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000270055900001},
      doi          = {10.1029/2008JD011369},
      url          = {https://juser.fz-juelich.de/record/4707},
}