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@ARTICLE{Tilmes:47476,
author = {Tilmes, S. and Müller, R. and Grooß, J.-U. and Spang, R.
and Sugitta, T. and Nakajima, H. and Sasano, Y.},
title = {{C}hemical ozone loss and related processes in the
{A}ntarctic winter 2003 based on {ILAS}-{II} observations},
journal = {Journal of Geophysical Research},
volume = {111},
issn = {0148-0227},
address = {Washington, DC},
publisher = {Union},
reportid = {PreJuSER-47476},
pages = {D11S12},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {In this study, ILAS-II (Improved Limb Atmospheric
Spectrometer) measurements were used to analyze chemical
ozone loss during the entire Antarctic winter 2003, using
the tracer-tracer correlation technique. The temporal
evolution of both the accumulated local chemical ozone loss
and the loss in column ozone in the lower stratosphere is in
step with increasing solar illumination. Half of the entire
loss in column ozone of 157 DU occurred during September
2003. By the end of September 2003, almost the total amount
of ozone was destroyed between 380 and 470 K. Further, ozone
loss rates increased strongly during September for the
entire lower stratosphere. The values of accumulated ozone
loss and ozone loss rates are strongly dependent on
altitude. Once ozone loss is saturated during September,
especially at latitudes between 380 and 420 K, ozone loss
rates decrease, and accumulated ozone loss can no longer
increase. Moreover, at altitudes above 470 K, accumulated
ozone loss depends on the amount of PSCs occurring during
winter and spring. During September, ozone mixing ratios
show a large day to day variation. Box model simulations by
the Chemical Lagrangian Model of the Stratosphere (CLaMS)
show that this is a result of the different histories of the
observed air masses. Further, the box model supports the
general evolution of ozone loss values during September as a
result of the strong increase of halogen catalyzed ozone
destruction.},
keywords = {J (WoSType)},
cin = {ICG-I},
ddc = {550},
cid = {I:(DE-Juel1)VDB47},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000237447400001},
doi = {10.1029/2005JD006260},
url = {https://juser.fz-juelich.de/record/47476},
}