Home > Publications database > Cl-Electrosorption on Ag(100) - Lateral Interactions and Electrosorption Valency from Monte Carlo Simulations and Experiments > print

001     47589
005     20190625110513.0
024 7 _ |2 DOI
|a 10.1016/j.electacta.2005.03.057
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037 _ _ |a PreJuSER-47589
041 _ _ |a eng
082 _ _ |a 540
084 _ _ |2 WoS
|a Electrochemistry
100 1 _ |a Abou-Hamad, I.
|b 0
|0 P:(DE-HGF)0
245 _ _ |a Cl-Electrosorption on Ag(100) - Lateral Interactions and Electrosorption Valency from Monte Carlo Simulations and Experiments
260 _ _ |a New York, NY [u.a.]
|b Elsevier
|c 2005
300 _ _ |a 5518 - 5525
336 7 _ |a Journal Article
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336 7 _ |a Journal Article
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336 7 _ |a ARTICLE
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336 7 _ |a JOURNAL_ARTICLE
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336 7 _ |a article
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440 _ 0 |a Electrochimica Acta
|x 0013-4686
|0 1776
|y 28
|v 50
500 _ _ |a Record converted from VDB: 12.11.2012
520 _ _ |a We present Monte Carlo simulations using an equilibrium lattice-gas model for the electrosorption of Cl on Ag(100) single-crystal surfaces. Fitting the simulated isotherms to chronocoulometry experiments, we extract parameters such as the electrosorption valency gamma and the next-nearest-neighbor lateral interaction energy phi(nnn). Both coverage-dependent and coverage-independent gamma were previously studied, assuming a constant phi(nnn) [I. Abou Hamad, Th. Wandlowski, G. Brown, P.A. Rikvold, J. Electroanal. Chem. 554-555 (2003) 211]. Here, a self-consistent, entirely electrostatic picture of the lateral interactions with a coverage-dependent phi(nnn) is developed, and a relationship between phi(nnn) and gamma is investigated for Cl on Ag(1 0 0). (C) 2005 Elsevier Ltd. All rights reserved.
536 _ _ |a Materialien, Prozesse und Bauelemente für die Mikro- und Nanoelektronik
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588 _ _ |a Dataset connected to Web of Science
650 _ 7 |a J
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653 2 0 |2 Author
|a chlorine electrosorption
653 2 0 |2 Author
|a lateral interactions
653 2 0 |2 Author
|a electrosorption valency
653 2 0 |2 Author
|a chronocoulornetry
653 2 0 |2 Author
|a continuous phase transition
653 2 0 |2 Author
|a Monte Carlo simulation
700 1 _ |a Mitchel, S. J.
|b 1
|0 P:(DE-HGF)0
700 1 _ |a Wandlowski, Th.
|b 2
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700 1 _ |a Rikvold, P. A.
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700 1 _ |a Brown, G.
|b 4
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773 _ _ |a 10.1016/j.electacta.2005.03.057
|g Vol. 50, p. 5518 - 5525
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|0 PERI:(DE-600)1483548-4
|t Electrochimica acta
|v 50
|y 2005
|x 0013-4686
856 7 _ |u http://dx.doi.org/10.1016/j.electacta.2005.03.057
909 C O |o oai:juser.fz-juelich.de:47589
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914 1 _ |y 2005
915 _ _ |0 StatID:(DE-HGF)0010
|a JCR/ISI refereed
920 1 _ |k ISG-3
|l Institut für Grenzflächen und Vakuumtechnologien
|d 31.12.2006
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920 1 _ |k CNI
|l Center of Nanoelectronic Systems for Information Technology
|d 14.09.2008
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