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@ARTICLE{Bejan:48758,
author = {Bejan, I. and Abd El Aal, Y. and Barnes, I. and Benter, T.
and Bohn, B. and Wiesen, P. and Kleffmann, J.},
title = {{T}he photolysis of ortho-nitrophenols: {A} new gas phase
source of {HONO}},
journal = {Physical Chemistry Chemical Physics},
volume = {8},
issn = {1463-9076},
address = {Cambridge},
publisher = {RSC Publ.},
reportid = {PreJuSER-48758},
pages = {2028 - 2035},
year = {2006},
note = {Record converted from VDB: 12.11.2012},
abstract = {Formation of nitrous acid (HONO) in the gas phase has been
observed for the first time in a flow tube photoreactor upon
irradiation (lambda = 300-500 nm) of 2-nitrophenol and
methyl substituted derivatives using a selective and
sensitive instrument (LOPAP) for the detection of HONO.
Formation of HONO by heterogeneous NO2 photochemistry has
been excluded, since production of NO2 under the
experimental conditions is negligible. Variation of the
surface to volume ratio and the nitrophenol concentration
showed that the photolysis occurred in the gas phase
indicating that HONO formation is initiated by
intramolecular hydrogen transfer from the phenolic OH group
to the nitro group. From the measured linear dependence of
the HONO formation rate on the reactant's concentration and
photolysis light intensity, a non-negligible new HONO source
is proposed for the urban atmosphere during the day.
Unexpectedly high HONO mixing ratios have been observed
recently in several field campaigns during the day. It is
proposed that the photolysis of aromatic compounds
containing the ortho-nitrophenol entity could help to
explain, at least in part, this high contribution of HONO to
the oxidation capacity of the urban atmosphere.},
keywords = {J (WoSType)},
cin = {ICG-II},
ddc = {540},
cid = {I:(DE-Juel1)VDB48},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Chemistry, Physical / Physics, Atomic, Molecular $\&$
Chemical},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:16633690},
UT = {WOS:000236970300006},
doi = {10.1039/b516590c},
url = {https://juser.fz-juelich.de/record/48758},
}