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@ARTICLE{Kim:4889,
author = {Kim, S. K. and Hoffmann-Eifert, S. and Mi, S. and Waser,
R.},
title = {{L}iquid injection atomic layer deposition of crystalline
{T}i{O}2 thin films with a smooth morphology from
{T}i({O}-i-{P}r)2({DPM})2},
journal = {Journal of the Electrochemical Society},
volume = {156},
issn = {0013-4651},
address = {Pennington, NJ},
publisher = {Electrochemical Society},
reportid = {PreJuSER-4889},
pages = {D296 - D300},
year = {2009},
note = {Record converted from VDB: 12.11.2012},
abstract = {TiO2 thin films were grown at susceptor temperatures from
340 to 470 degrees C by liquid injection atomic layer
deposition (ALD) using Ti(O-i-Pr)(2)(DPM)(2)
[Ti(OC3H7)(2)(C11H19O2)(2), titanium dipivaloylmethanato
di-isopropoxide] dissolved in ethylcyclohexane as a Ti
source and H2O as an oxidant. The self-saturation growth
behavior of the TiO2 films was confirmed up to 390 degrees
C. Within the ALD window, the growth rate of the films
increased from 0.022 nm/cycle at 340 degrees C to 0.046
nm/cycle at 390 degrees C, and the films exhibited a carbon
content below 3 atom $\%.$ Due to the thermal decomposition
of the precursor at 470 degrees C, the growth rate of the
films largely increased and the film density decreased by
the increase in the carbon content of the film. The films
showed quite a smooth surface morphology over the whole
range of growth temperatures. The increase in the film
thickness did not significantly change the surface
morphology of the films due to the formation of the
crystalline phase even at an initial growth stage. The
relative permittivity of the TiO2 films, which were
crystallized into an anatase structure, was approximately
35-40. The films grown within the ALD window showed
reasonable leakage current properties.},
keywords = {J (WoSType)},
cin = {IFF-6 / IFF-8 / JARA-FIT},
ddc = {540},
cid = {I:(DE-Juel1)VDB786 / I:(DE-Juel1)VDB788 /
$I:(DE-82)080009_20140620$},
pnm = {Grundlagen für zukünftige Informationstechnologien},
pid = {G:(DE-Juel1)FUEK412},
shelfmark = {Electrochemistry / Materials Science, Coatings $\&$ Films},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000267798500041},
doi = {10.1149/1.3138722},
url = {https://juser.fz-juelich.de/record/4889},
}