%0 Journal Article %A Mironov, V. P. %A Matusevich, J. L. %A Kudrjashov, V. P. %A Ananich, P. I. %A Zhuravkov, V. V. %A Boulyga, S. F. %A Becker, J. S. %T Determination of uranium concentration and burn-up of irradiated reactor fuel in contaminated areas in Belarus using uranium isotopic ratios in soil samples %J Radiochimica acta %V 93 %@ 0033-8230 %C München %I Oldenbourg %M PreJuSER-49535 %P 781 - 784 %D 2005 %Z Record converted from VDB: 12.11.2012 %X An analytical method is described for the estimation of uranium concentrations, of U-235/U-238 and U-236/U-238 isotope ratios and burn-up of irradiated reactor uranium in contaminated soil samples by inductively coupled plasma mass spectrometry. Experimental results obtained at 12 sampling sites situated on northern and western radioactive fallout tails 4 to 53 km distant from Chernobyl nuclear power plant (NPP) are presented. Concentrations of irradiated uranium in the upper 0-10cm soil layers at the investigated sampling sites varied from 2.1 x 10(-9) g/g to 2.0 x 10(-6) /g depending mainly on the distance from Chernobyl NPP. A slight variation of the degree of burn-up of spent reactor uranium was revealed by analyzing U-235/U-238 U and U-236/U-211 isotope ratios and the average value amounted to 9.4 +/- 0.3 MWd/(kg, U). %K J (WoSType) %F PUB:(DE-HGF)16 %9 Journal Article %U <Go to ISI:>//WOS:000234479900008 %R 10.1524/ract.2005.93.12.781 %U https://juser.fz-juelich.de/record/49535