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@ARTICLE{Schlosser:49896,
author = {Schlosser, E. and Bohn, B. and Brauers, T. and Dorn, H. P.
and Fuchs, H. and Häseler, R. and Hofzumahaus, A. and
Holland, F. and Rohrer, F. and Rupp, L. and Siese, M. and
Tillmann, R. and Wahner, A.},
title = {{I}ntercomparison of {T}wo {H}ydroxyl {R}adical
{M}easurement {T}echniques at the {A}tmosphere {S}imulation
{C}hamber {SAPHIR}},
journal = {Journal of atmospheric chemistry},
volume = {56},
issn = {0167-7764},
address = {Dordrecht [u.a.]},
publisher = {Springer Science + Business Media B.V},
reportid = {PreJuSER-49896},
pages = {187 - 205},
year = {2007},
note = {Record converted from VDB: 12.11.2012},
abstract = {At the atmosphere simulation chamber SAPHIR in Julich both
Laser-Induced Fluorescence Spectroscopy (LIF) and Long-Path
Differential Optical Laser Absorption Spectroscopy (DOAS)
are operational for the detection of OH radicals at
tropospheric levels. The two different spectroscopic
techniques were compared within the controlled environment
of SAPHIR based on all simultaneous measurements acquired in
2003 ( 13 days). Hydroxyl radicals were scavenged by added
CO during four of these days in order to experimentally
check the calculated precisions at the detection limit. LIF
measurements have a higher precision (sigma = 0.88 x 10(6)
cm(-3)) and better time resolution (Delta t = 60 s), but the
DOAS method (sigma = 1.24 x 10(6) cm(-3), Delta t = 135 s)
is regarded as primary standard for comparisons because of
its good accuracy. A high correlation coefficient of r =
0.95 was found for the whole data set highlighting the
advantage of using a simulation chamber. The data set
consists of two groups. The first one includes 3 days, where
the LIF measurements yield ( 1 2) x 10(6) cm(-3) higher OH
concentrations than observed by the DOAS instrument. The
experimental conditions during these days are characterized
by increased NOx concentration and a small dynamic range in
OH. Excellent agreement is found within the other group of 6
days. The regression to the combined data of this large
group yields unity slope without a significant offset.},
keywords = {J (WoSType)},
cin = {ICG-2 / JARA-ENERGY / JARA-SIM},
ddc = {540},
cid = {I:(DE-Juel1)VDB791 / $I:(DE-82)080011_20140620$ /
I:(DE-Juel1)VDB1045},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK406},
shelfmark = {Environmental Sciences / Meteorology $\&$ Atmospheric
Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000244187300005},
doi = {10.1007/s10874-006-9049-3},
url = {https://juser.fz-juelich.de/record/49896},
}