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@ARTICLE{Anttila:50162,
      author       = {Anttila, T. and Vehkamäki, H. and Napari, I. and Kulmala,
                      M.},
      title        = {{E}ffect of ammonium bisulphate formation on atmospheric
                      water-sulphuric acid-ammonia nucleation},
      journal      = {Boreal environment research},
      volume       = {10},
      issn         = {1239-6095},
      address      = {Helsinki},
      publisher    = {Finnish Zoological and Botanical Publishing Board},
      reportid     = {PreJuSER-50162},
      pages        = {511 - 523},
      year         = {2005},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {The effect of formation of stable ammonium bisulphate
                      clusters on the ternary water-sulphuric acid-ammonia
                      nucleation was investigated by means of the classical
                      thermodynamics. The performed calculations show that most of
                      the sulphuric acid in the atmosphere is likely to be bound
                      to stable ammonium bisulphate clusters. Consequently the
                      nucleation rates calculated with the new model are orders,
                      sometimes even tens of orders, of magnitude lower than the
                      rates produced by the previous ternary model which neglected
                      the formation of these clusters. The new nucleation rates
                      compare favourably with the available experimental results,
                      unlike the old ones, which are far too high. In contrast to
                      the old ternary model, the revised model does not predict
                      significant nucleation rates that would explain new particle
                      formation events every time they are observed, and we have
                      to look for other nucleation mechanisms like multi-component
                      nucleation involving organics or ion induced nucleation to
                      understand atmospheric new particle formation.},
      keywords     = {J (WoSType)},
      cin          = {ICG-II},
      ddc          = {333.7},
      cid          = {I:(DE-Juel1)VDB48},
      pnm          = {Chemie und Dynamik der Geo-Biosphäre},
      pid          = {G:(DE-Juel1)FUEK257},
      shelfmark    = {Environmental Sciences},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000234227300004},
      url          = {https://juser.fz-juelich.de/record/50162},
}