TY - JOUR
AU - Elter, P.
AU - Eckold, G.
AU - Gibhardt, H.
AU - Schmidt, W.
AU - Hoser, A.
TI - Kinetics of decomposition in ionic solids: IV: Transition between nucleation and spinodal decomposition observed by time-resolved phonon spectroscopy
JO - Journal of physics / Condensed matter
VL - 17
SN - 0953-8984
CY - Bristol
PB - IOP Publ.
M1 - PreJuSER-51540
SP - 6559 - 6573
PY - 2005
N1 - Record converted from VDB: 12.11.2012
AB - Real-time inelastic neutron scattering has been used to study the kinetics of the demixing process in AgBr-NaBr mixed single crystals. The variation of transverse acoustic phonon spectra provides most direct information about the microscopic non-equilibrium behaviour. The phase separation is monitored by a well defined splitting of phonon peaks that reflects the different dynamical behaviours of the constituents. As a function of temperature, time evolution of the phonon spectra changes drastically, thus proving unambiguously that the demixing process is dominated by nucleation in the high-temperature regime and by concentration fluctuations at low temperatures.
KW - J (WoSType)
LB - PUB:(DE-HGF)16
UR - <Go to ISI:>//WOS:000233589400030
DO - DOI:10.1088/0953-8984/17/41/025
UR - https://juser.fz-juelich.de/record/51540
ER -